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@ARTICLE{Schlautmann:1041123,
      author       = {Schlautmann, Eva and Drews, Janina and Ketter, Lukas and
                      Lange, Martin A. and Danner, Timo and Latz, Arnulf and
                      Zeier, Wolfgang},
      title        = {{G}raded {C}athode {D}esign for {E}nhanced {P}erformance of
                      {S}ulfide-{B}ased {S}olid-{S}tate {B}atteries},
      journal      = {ACS energy letters},
      volume       = {10},
      issn         = {2380-8195},
      address      = {Washington, DC},
      publisher    = {American Chemical Society},
      reportid     = {FZJ-2025-02157},
      pages        = {1664 - 1670},
      year         = {2025},
      note         = {Financial support by the German Federal Ministry of
                      Research and Education (BMBF) within the scope of the
                      Cluster of Competence for Solid State Batteries FestBatt2
                      (FKZ: 03XP0435A) and ANISSA (FKZ: 05K22PMA)},
      abstract     = {Solid-state batteries present a promising technology to
                      overcome the energy density limitations of lithium-ion
                      batteries. However, achieving a high areal loading in
                      cathodes without introducing significant transport
                      limitations remains a key challenge, particularly in thick
                      electrodes. In this work, we study the impact of a
                      three-layer graded cathode design on the performance of a
                      $LiNi_{0.83}Co_{0.11}Mn_{0.06}O_2$ (NCM83)$/ Li_6PS_5Cl$
                      (LPSCl) composite cathode using a combination of experiments
                      and microstructure-resolved simulations. An increased LPSCl
                      content at the separator and higher NCM83 content toward the
                      current collector improve effective charge transport,
                      resulting in better rate performance and reduced
                      overpotentials at high current densities. This comprehensive
                      experimental and theoretical study demonstrates that the
                      optimization of cathode design has the potential to
                      significantly enhance the performance of solid-state
                      batteries.},
      cin          = {IMD-4},
      ddc          = {333.7},
      cid          = {I:(DE-Juel1)IMD-4-20141217},
      pnm          = {1222 - Components and Cells (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1222},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:001444249700001},
      doi          = {10.1021/acsenergylett.4c03243},
      url          = {https://juser.fz-juelich.de/record/1041123},
}