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@ARTICLE{Tilgner:1041523,
author = {Tilgner, Niclas and Wolff, Susanne and Soubatch, Serguei
and Lee, Tien-Lin and Göhler, Fabian and Tautz, Frank
Stefan and Seyller, Thomas and Schädlich, Philip and Kumpf,
Christian},
title = {{S}olving the {P}hase {P}roblem of {D}iffraction:{X}-ray
{S}tanding {W}aves {I}maging on {B}ismuthene/{S}i{C}(0001)},
reportid = {FZJ-2025-02297},
year = {2025},
abstract = {The phase retrieval problem is a fundamental shortcoming of
all diffraction-based methods, arising from theinability to
measure the phase of scattered waves. The (normal incidence)
X-ray standing wave (NIXSW) techniquecircumvents this issue
by introducing a (Bragg-generated) X-ray standing wave field
throughout the sample, rela-tive to which any atomic species
can be localized by probing its fluorescence or
photoelectron yield. In essence,in a single measurement the
complex scattering factor (i.e., its amplitude and phase)
corresponding to the usedBragg reflection is determined.
Performing this for multiple Bragg reflections enables one
to reconstruct the scat-tering density of the sample in
three dimensions, straightforwardly as the Fourier sum of
all measured (complex)scattering factors. Here, we utilize
this technique to reveal the structural key features
involved in the formation ofthe quantum spin Hall insulator
bismuthene on silicon carbide. In this prominent example,
the two-dimensional Bilayer is confined between a 4H-SiC
substrate crystal and an epitaxial graphene layer. The key
finding is a changein the adsorption site of the Bi atoms
underneath the graphene upon hydrogenation, caused by the
H-saturation ofone (out of three) Si dangling bonds per unit
cell. This structural change, clearly revealed by our NIXSW
imagingexperiment, is the key feature leading to the
formation of the characteristic band structure of the 2D
bismuthenehoneycomb.},
cin = {PGI-3},
cid = {I:(DE-Juel1)PGI-3-20110106},
pnm = {5213 - Quantum Nanoscience (POF4-521) / SFB 1083 A12 -
Struktur und Anregungen von hetero-epitaktischen
Schichtsystemen aus schwach wechselwirkenden 2D-Materialien
und molekularen Schichten (A12) (385975694)},
pid = {G:(DE-HGF)POF4-5213 / G:(GEPRIS)385975694},
typ = {PUB:(DE-HGF)25},
doi = {10.48550/arXiv.2504.11413},
url = {https://juser.fz-juelich.de/record/1041523},
}