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@ARTICLE{MartinezCastro:1041579,
author = {Martinez-Castro, Jose and Bolat, Rustem and Fan, Qitang and
Werner, Simon and Arefi, Hadi and Esat, Taner and
Sundermeyer, Jörg and Wagner, Christian and Gottfried, J.
Michael and Temirov, Ruslan and Ternes, Markus and Tautz, F.
Stefan},
title = {{D}isentangling the {C}omplex {E}lectronic {S}tructure of
an {A}dsorbed {N}anographene: {C}ycloarene {C}108},
publisher = {arXiv},
reportid = {FZJ-2025-02318},
year = {2021},
abstract = {We combine low-temperature scanning tunneling spectroscopy,
CO functionalized tips and algorithmic data analysis to
investigate the electronic structure of the molecular
cycloarene C108 (graphene nanoring) adsorbed on a Au(111)
surface. We demonstrate that CO functionalized tips enhance
the visibility of molecular resonances, both in differential
conductance spectra and in real-space topographic images
without introducing spurious artifacts. Comparing our
experimental data with ab-initio density functional theory
reveals a remarkably precise agreement of the molecular
orbitals and enables us to disentangle close-lying molecular
states only separated by 50 meV at an energy of 2 eV below
the Fermi level. We propose this combination of techniques
as a promising new route for a precise characterization of
complex molecules and other physical entities which have
electronic resonances in the tip-sample junction.},
keywords = {Mesoscale and Nanoscale Physics (cond-mat.mes-hall) (Other)
/ FOS: Physical sciences (Other)},
cin = {PGI-3},
cid = {I:(DE-Juel1)PGI-3-20110106},
pnm = {5213 - Quantum Nanoscience (POF4-521)},
pid = {G:(DE-HGF)POF4-5213},
typ = {PUB:(DE-HGF)25},
doi = {10.48550/ARXIV.2110.11449},
url = {https://juser.fz-juelich.de/record/1041579},
}