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001041721 1001_ $$0P:(DE-HGF)0$$aTaoussi, S.$$b0$$eCorresponding author
001041721 245__ $$aInsights into structural, thermal, physical, optical, and electrical properties of novel ZnO-doped lithium–titanium-phosphate glasses
001041721 260__ $$aNew York, NY [u.a.]$$bElsevier$$c2025
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001041721 520__ $$aThis study investigates novel ZnO-doped lithium-titanium-phosphate glasses, synthesized via the melt-quenching method, and characterizes their physical, structural, thermal, optical, chemical, mechanical, and electrical properties, with a focus on the impact of varying ZnO content on these properties. An increase in ZnO content from 20 mol% to 27.27 mol% induces significant local structural changes, promoting enhanced network polymerization, density, and chemical durability, while concurrently reducing thermal stability and mechanical strength. EPR analysis confirmed that titanium remained in the Ti4+ state, while optical measurements revealed an increased band gap, attributed to the role of ZnO in preventing Ti4+ reduction and minimizing localized states. The electrical conductivity decreases with increasing ZnO content, with the highest value measured at 1.73 × 10-10 Ω-1 cm-1. High-ZnO glasses exhibit mainly electronic conductivity of 4.02 × 10-9 Ω-1 cm-1 at room temperature. The frequency-dependent conductivity follows Jonscher's power law, with the charge transport governed by a correlated barrier-hopping mechanism, remaining stable across temperatures and compositions.
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001041721 7001_ $$0P:(DE-HGF)0$$aOuaha, A.$$b1
001041721 7001_ $$0P:(DE-HGF)0$$aNaji, M.$$b2
001041721 7001_ $$0P:(DE-HGF)0$$aHoummada, K.$$b3
001041721 7001_ $$0P:(DE-HGF)0$$aLahmar, A.$$b4
001041721 7001_ $$0P:(DE-HGF)0$$aCailleu, D.$$b5
001041721 7001_ $$00000-0002-4919-5350$$aAlami, J.$$b6
001041721 7001_ $$0P:(DE-HGF)0$$aManoun, B.$$b7
001041721 7001_ $$0P:(DE-HGF)0$$aEl bouari, A.$$b8
001041721 7001_ $$0P:(DE-Juel1)130646$$aFrielinghaus, H.$$b9$$ufzj
001041721 7001_ $$0P:(DE-HGF)0$$aBih, L.$$b10
001041721 773__ $$0PERI:(DE-600)1491959-X$$a10.1016/j.matchemphys.2025.130468$$gVol. 334, p. 130468 -$$p130468$$tMaterials chemistry and physics$$v334$$x0254-0584$$y2025
001041721 8564_ $$uhttps://juser.fz-juelich.de/record/1041721/files/Insights%20into%20Structural%2C%20Thermal%2C%20Physical%2C%20Optical%2C%20and%20Electrical%20Properties%20of%20Novel%20ZnO-Doped%20Lithium-Titanium-Phosphate%20Glasses.pdf$$yPublished on 2025-01-31. Available in OpenAccess from 2027-01-31.
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