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001043689 1001_ $$00009-0001-7592-7674$$aTilgner, Niclas$$b0$$eFirst author
001043689 245__ $$aReversible switching of the environment-protected quantum spin Hall insulator bismuthene at the graphene/SiC interface
001043689 260__ $$a[London]$$bSpringer Nature$$c2025
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001043689 520__ $$aQuantum spin Hall insulators have been extensively studied both theoretically and experimentally because they exhibit robust helical edge states driven by spin-orbit coupling and offer the potential for applications in spintronics through dissipationless spin transport. Here we show that a single layer of elemental Bi, formed by intercalation of an epitaxial graphene buffer layer on SiC(0001), is a promising candidate for a quantum spin Hall insulator. This layer can be reversibly switched between an electronically inactive precursor state and a bismuthene state, the latter exhibiting the predicted band structure of a true two-dimensional bismuthene layer. Switching is accomplished by hydrogenation (dehydrogenation) of the sample. A partial passivation (activation) of Si dangling bonds causes a lateral shift of Bi atoms involving a change of the adsorption site. In the bismuthene state, the Bi honeycomb layer is a prospective quantum spin Hall insulator, inherently protected by the graphene sheet above and the H-passivated substrate below.
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001043689 536__ $$0G:(GEPRIS)385975694$$aSFB 1083 A12 - Struktur und Anregungen von hetero-epitaktischen Schichtsystemen aus schwach wechselwirkenden 2D-Materialien und molekularen Schichten (A12) (385975694)$$c385975694$$x2
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001043689 7001_ $$00009-0003-6480-9319$$aWolff, Susanne$$b1
001043689 7001_ $$0P:(DE-Juel1)128790$$aSoubatch, Serguei$$b2
001043689 7001_ $$00000-0001-6935-5983$$aLee, Tien-Lin$$b3
001043689 7001_ $$00009-0002-3283-5283$$aPeña Unigarro, Andres David$$b4
001043689 7001_ $$00000-0003-0455-1945$$aGemming, Sibylle$$b5
001043689 7001_ $$0P:(DE-Juel1)128791$$aTautz, F. Stefan$$b6
001043689 7001_ $$00000-0002-4953-2142$$aSeyller, Thomas$$b7
001043689 7001_ $$0P:(DE-Juel1)128774$$aKumpf, Christian$$b8$$eCorresponding author
001043689 7001_ $$00000-0003-2299-2445$$aGöhler, Fabian$$b9$$eCorresponding author
001043689 7001_ $$00000-0002-0075-2291$$aSchädlich, Philip$$b10$$eCorresponding author
001043689 773__ $$0PERI:(DE-600)2553671-0$$a10.1038/s41467-025-60440-x$$gVol. 16, no. 1, p. 6171$$n1$$p6171$$tNature Communications$$v16$$x2041-1723$$y2025
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