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@ARTICLE{Heinze:1044510,
author = {Heinze, Leonie and Kotte, T. and Rausch, R. and Demuer, A.
and Luther, S. and Feyerherm, R. and Ammerlaan, E. L. Q. N.
and Zeitler, U. and Gorbunov, D. I. and Uhlarz, M. and Rule,
K. C. and Wolter, A. U. B. and Kühne, H. and Wosnitza, J.
and Karrasch, C. and Süllow, S.},
title = {{A}tacamite {C}u$_2${C}l({OH})$_3$ in {H}igh {M}agnetic
{F}ields: {Q}uantum {C}riticality and {D}imensional
{R}eduction of a {S}awtooth-{C}hain {C}ompound},
journal = {Physical review letters},
volume = {134},
number = {21},
issn = {0031-9007},
address = {College Park, Md.},
publisher = {APS},
reportid = {FZJ-2025-03247},
pages = {216701},
year = {2025},
abstract = {We report an extensive high-field study of atacamite
Cu$_2$Cl(OH)$_3$, a material realization of quantum
sawtooth chains with weak interchain couplings, in
continuous and pulsed magnetic fields up to 58 T. In
particular, we have mapped the entropy landscape for fields
as high as 35 T and have identified a field-induced quantum
critical point at 21.9(1) T for H || c axis. The quantum
critical point separates field regions with and without
magnetic order, evidenced by our thermodynamic study and
$^1$H nuclear magnetic resonance spectroscopy, but lies far
below full saturation of the magnetization. Corroborated by
numerical results using density-matrix renormalization group
calculations, we find this behavior associated with a
dimensional reduction of the spin system: the sawtooth chain
effectively decouples into an antiferromagnetic spin-1/2
chain (backbone of the sawtooth chain) in the presence of an
exchange field produced by the remaining field-polarized
spins.},
cin = {JCNS-4 / JCNS-3 / MLZ / JCNS-FRM-II},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-4-20201012 / I:(DE-Juel1)JCNS-3-20170926 /
I:(DE-588b)4597118-3 / I:(DE-Juel1)JCNS-FRM-II-20110218},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (FZJ)
(POF4-6G4) / 632 - Materials – Quantum, Complex and
Functional Materials (POF4-632)},
pid = {G:(DE-HGF)POF4-6G4 / G:(DE-HGF)POF4-632},
experiment = {EXP:(DE-MLZ)NOSPEC-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {40531025},
UT = {WOS:001503644200008},
doi = {10.1103/PhysRevLett.134.216701},
url = {https://juser.fz-juelich.de/record/1044510},
}