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@PHDTHESIS{Abuawad:1044576,
author = {Abuawad, Abdalhalim},
title = {{D}evelopment of {S}uperparamagnetic {B}ased {B}iological
{S}ensor for the {D}etection of {B}rucella {DNA} {U}sing
{F}requency {M}ixing {M}agnetic {D}etection},
volume = {113},
school = {RWTH Aachen University},
type = {Dissertation},
address = {Jülich},
publisher = {Forschungszentrum Jülich GmbH Zentralbibliothek, Verlag},
reportid = {FZJ-2025-03256},
isbn = {978-3-95806-836-0},
series = {Schriften des Forschungszentrums Jülich Reihe Information
/ Information},
pages = {X, 129},
year = {2025},
note = {Dissertation, RWTH Aachen University, 2025},
abstract = {Early detection of zoonotic diseases is essential in
preventing the consequences of outbreaks and reemergence
occurrences. Brucellosis is endemic in several countries and
has re-emerged with a high prevalence rate in different
locations, affecting livestock and public health sectors.
Due to the limitations of conventional Brucella detection
methods, including limited specificity, long incubation
times and safety concerns, developing a rapid, selective and
accurate technique for the early detection of Brucella in
livestock animals is crucial to prevent the spread of the
associated disease. In the present thesis, we introduce a
magnetic nanoparticle marker-based biosensor using Frequency
Mixing Magnetic Detection (FMMD) for the detection and
quantification of Brucella DNA. Magnetic nanoparticles
(MNPs) were used as magnetically measured markers to
selectively detect the target DNA hybridized with its
complementary capture probes immobilized on a porous
polyethylene filter. Our sensor demonstrated a relatively
fast detection time of approximately 10 min, with a
detection limit of 0.09 fM when tested using DNA amplified
from Brucella genetic material by means of Polymerase Chain
Reaction (PCR). In addition, the detection specificity was
examined using gDNA from Brucella and other zoonotic
bacteria that may coexist in the same niche, confirming the
method’s selectivity for Brucella DNA. To enhance the
practicality of the developed assay, we combined it with
isothermal Recombinase Polymerase Amplification (RPA) and
achieved rapid detection of 9 fM Brucella DNA in 25 minutes
total assay time. In addition to isothermal DNA
amplification in a water bath, we showed the feasibility of
RPA directly inside our portable FMMD-based device. When
being controlled by means of pulse width modulation (PWM),
the inherently generated heat of the low frequency (LF)
excitation coil of the magnetic reader can be utilized to
serve as a constant temperature bath for RPA, thus enabling
isothermal amplification inside the magnetic measurement
head. We confirmed that RPA performs with high efficiency in
the sensor unit of the FMMD device. In summary, the
portability of the measurement device, the selective sensing
of MNPs, the fast detection time, and the ability to deliver
quantitative results make this biosensor a valuable tool for
early on-site diagnosis and monitoring of Brucella
infections in resource-limited settings.},
cin = {IBI-3},
cid = {I:(DE-Juel1)IBI-3-20200312},
pnm = {5241 - Molecular Information Processing in Cellular Systems
(POF4-524)},
pid = {G:(DE-HGF)POF4-5241},
typ = {PUB:(DE-HGF)3 / PUB:(DE-HGF)11},
urn = {urn:nbn:de:0001-2508151006385.053377491913},
doi = {10.34734/FZJ-2025-03256},
url = {https://juser.fz-juelich.de/record/1044576},
}