% IMPORTANT: The following is UTF-8 encoded. This means that in the presence
% of non-ASCII characters, it will not work with BibTeX 0.99 or older.
% Instead, you should use an up-to-date BibTeX implementation like “bibtex8” or
% “biber”.
@ARTICLE{Wu:1044611,
author = {Wu, Jianchang and Hu, Manman and Dai, Qingqing and Alkan,
Ecem Aydan and Barabash, Anastasia and Zhang, Jiyun and Liu,
Chao and Hauch, Jens and Han, Gao-Feng and Jiang, Qing and
Wang, Tonghui and Seok, Sang Il and Brabec, Christoph},
title = {{H}ighly {S}table {S}n─{P}b {P}erovskite {S}olar {C}ells
{E}nabled by {P}henol‐{F}unctionalized {H}ole
{T}ransporting {M}aterial},
journal = {Angewandte Chemie / International edition},
volume = {64},
number = {22},
issn = {1433-7851},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2025-03282},
pages = {e202424515},
year = {2025},
abstract = {Sn─Pb perovskites, a most promising low bandgap
semiconductor for multi-junction solar cells, are often
limited by instability due to the susceptibility of Sn2+ to
oxidation. Inspired by the antioxidative properties of
polyphenolic compounds, we introduce the reductive phenol
group and strong electronegative fluorine into an organic
conjugated structure and design a multi-functional polymer
with fluorine and phenol units (PF─OH). The design of
PF─OH allows the effective rise in the energy barrier of
Sn2+ oxidation, leading to a significant enhancement in the
stability of Sn─Pb perovskite devices from 200 to 8000
h—an improvement of around 100 times. Additionally, the
strong binding energy between Sn2+ and the phenol in PF─OH
critically influences Sn─Pb perovskite's crystallization
and grain growth, resulting in perovskite films with fewer
pinholes at the buried interface and extended carrier
lifetimes. This enhancement not only boosts the power
conversion efficiency (PCE) to $23.61\%,$ but also
significantly improves the operational stability of the
devices. Ultimately, this design strategy has been proven
universal through the phenolization of a series of
molecules, marking a milestone in enhancing the stability of
Sn─Pb perovskites.},
cin = {IET-2},
ddc = {540},
cid = {I:(DE-Juel1)IET-2-20140314},
pnm = {1213 - Cell Design and Development (POF4-121)},
pid = {G:(DE-HGF)POF4-1213},
typ = {PUB:(DE-HGF)16},
pubmed = {40127212},
UT = {WOS:001457461700001},
doi = {10.1002/anie.202424515},
url = {https://juser.fz-juelich.de/record/1044611},
}