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001044673 1001_ $$0P:(DE-HGF)0$$aPeng, Zijian$$b0$$eCorresponding author
001044673 245__ $$aLocating Non‐Radiative Recombination Losses and Understanding Their Impact on the Stability of Perovskite Solar Cells During Photo‐Thermal Accelerated Ageing
001044673 260__ $$aWeinheim$$bWiley-VCH$$c2025
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001044673 520__ $$aCommercialization of perovskite solar cells (PSCs) requires further breakthroughs in stability, but the complex degradation mechanisms and the interplay of the underlying stress factors complicate insight-driven improvement of long-term stability. This study establishes a quantitative link between potential degradation—specifically open-circuit voltage (VOC) and quasi-Fermi level splitting (QFLS)—and the photo-thermal stability of PSCs. It is highlighted that an increase in non-radiative recombination losses induces the seemingly negligible decrease in VOC and QFLS, though it causes a significant decrease in fill factor (FF) and/or short circuit current (JSC) instead, leading to an overall performance decline. By combining non-destructive photoluminescence imaging and drift-diffusion simulations, it is revealed that during photo-thermal ageing, unstable low-dimensional passivation fails within tens of hours, generating bulk defects, while unstable hole-transport-layer contacts induce interface defects within hours. Building on these findings, a robust hole-transport-layer polymer interface is employed and enhanced perovskite crystal quality to suppress both interface and bulk defect generation during ageing, achieving a T80 lifetime exceeding 1000 h under accelerated ageing conditions (85 °C and two-sun illumination).
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001044673 7001_ $$0P:(DE-Juel1)196016$$aWortmann, Jonas$$b1
001044673 7001_ $$0P:(DE-HGF)0$$aHong, Jisu$$b2
001044673 7001_ $$0P:(DE-HGF)0$$aZhou, Shuyu$$b3
001044673 7001_ $$0P:(DE-HGF)0$$aBornschlegl, Andreas J.$$b4
001044673 7001_ $$0P:(DE-Juel1)207892$$aHaffner-Schirmer, Julian$$b5$$ufzj
001044673 7001_ $$0P:(DE-HGF)0$$aCorre, Vincent M. Le$$b6
001044673 7001_ $$0P:(DE-Juel1)180635$$aHeumüller, Thomas$$b7
001044673 7001_ $$0P:(DE-HGF)0$$aOsvet, Andres$$b8
001044673 7001_ $$0P:(DE-HGF)0$$aRand, Barry P.$$b9
001044673 7001_ $$0P:(DE-Juel1)206674$$aLüer, Larry$$b10$$eCorresponding author
001044673 7001_ $$0P:(DE-Juel1)176427$$aBrabec, Christoph J.$$b11$$eCorresponding author
001044673 773__ $$0PERI:(DE-600)2594556-7$$a10.1002/aenm.202502787$$gp. 2502787$$n35$$p2502787$$tAdvanced energy materials$$v15$$x1614-6832$$y2025
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