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| 100 | 1 | _ | |a Peng, Zijian |0 P:(DE-HGF)0 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Locating Non‐Radiative Recombination Losses and Understanding Their Impact on the Stability of Perovskite Solar Cells During Photo‐Thermal Accelerated Ageing |
| 260 | _ | _ | |a Weinheim |c 2025 |b Wiley-VCH |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Commercialization of perovskite solar cells (PSCs) requires further breakthroughs in stability, but the complex degradation mechanisms and the interplay of the underlying stress factors complicate insight-driven improvement of long-term stability. This study establishes a quantitative link between potential degradation—specifically open-circuit voltage (VOC) and quasi-Fermi level splitting (QFLS)—and the photo-thermal stability of PSCs. It is highlighted that an increase in non-radiative recombination losses induces the seemingly negligible decrease in VOC and QFLS, though it causes a significant decrease in fill factor (FF) and/or short circuit current (JSC) instead, leading to an overall performance decline. By combining non-destructive photoluminescence imaging and drift-diffusion simulations, it is revealed that during photo-thermal ageing, unstable low-dimensional passivation fails within tens of hours, generating bulk defects, while unstable hole-transport-layer contacts induce interface defects within hours. Building on these findings, a robust hole-transport-layer polymer interface is employed and enhanced perovskite crystal quality to suppress both interface and bulk defect generation during ageing, achieving a T80 lifetime exceeding 1000 h under accelerated ageing conditions (85 °C and two-sun illumination). |
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| 700 | 1 | _ | |a Wortmann, Jonas |0 P:(DE-Juel1)196016 |b 1 |
| 700 | 1 | _ | |a Hong, Jisu |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Zhou, Shuyu |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Bornschlegl, Andreas J. |0 P:(DE-HGF)0 |b 4 |
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| 700 | 1 | _ | |a Osvet, Andres |0 P:(DE-HGF)0 |b 8 |
| 700 | 1 | _ | |a Rand, Barry P. |0 P:(DE-HGF)0 |b 9 |
| 700 | 1 | _ | |a Lüer, Larry |0 P:(DE-Juel1)206674 |b 10 |e Corresponding author |
| 700 | 1 | _ | |a Brabec, Christoph J. |0 P:(DE-Juel1)176427 |b 11 |e Corresponding author |
| 773 | _ | _ | |a 10.1002/aenm.202502787 |g p. 2502787 |0 PERI:(DE-600)2594556-7 |n 35 |p 2502787 |t Advanced energy materials |v 15 |y 2025 |x 1614-6832 |
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