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@ARTICLE{Holka:10454,
author = {Holka, F. and Szalay, P.G. and Müller, T. and Tyuterev,
V.G.},
title = {{T}oward an {I}mproved {G}round {S}tate {P}otential
{E}nergy {S}urface of {O}zone},
journal = {The journal of physical chemistry / A},
volume = {114},
issn = {1089-5639},
address = {Washington, DC},
publisher = {Soc.},
reportid = {PreJuSER-10454},
pages = {9927 - 9935},
year = {2010},
note = {We acknowledge the support from ANR "IDEO" and LEFE-CHAT
CNRS grants, from Balaton French-Hungarian PHC exchange
program and its Hungarian counterpart TeT, from IDRIS
computer centre of CNRS France and of the computer centre
Reims-Champagne-Ardenne. F. H. thanks the CNRS for the
postdoc support at University of Reims and for the
opportunity to work on this project. P. S. acknowledges
support by OTKA (grant number F72423). The support of VEGA
1/0648/10 is also acknowledged.},
abstract = {A systematic study of the ozone potential energy surface
was performed by means of high level ab initio techniques.
The methods include icMR-CISD and icMR-AQCC with all
electrons correlated using a full valence CAS reference
space and basis sets up to sextuple-ζ quality along with
extrapolation to the complete basis set limit. We computed a
dense 3D grid as well as 1D cuts along stretching and
bending coordinates around the open (C(2v)) equilibrium
structure as well as along the minimum energy path to
dissociation including the transition state and the van der
Waals minimum region. The detailed analysis of our results
confirms earlier calculations by the Schinke group and
assures that these are not biased by deficiencies of the
basis set, lack of relativistic corrections, or core
correlation effects. Finally, we discuss possible sources of
error that may explain the remaining discrepancies compared
to experimental findings.},
keywords = {J (WoSType)},
cin = {JSC},
ddc = {530},
cid = {I:(DE-Juel1)JSC-20090406},
pnm = {Scientific Computing (FUEK411) / 411 - Computational
Science and Mathematical Methods (POF2-411)},
pid = {G:(DE-Juel1)FUEK411 / G:(DE-HGF)POF2-411},
shelfmark = {Chemistry, Physical / Physics, Atomic, Molecular $\&$
Chemical},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:20825243},
UT = {WOS:000281567500041},
doi = {10.1021/jp104182q},
url = {https://juser.fz-juelich.de/record/10454},
}