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@ARTICLE{Guratinder:1045689,
author = {Guratinder, K. and Johnson, R. D. and Prabhakaran, D. and
Taylor, R. A. and Lang, F. and Blundell, S. J. and Taran, L.
S. and Streltsov, S. V. and Williams, T. J. and Giblin, S.
R. and Fennell, T. and Schmalzl, K. and Stock, C.},
title = {{M}agnetoelastic {D}ynamics of the {S}pin {J}ahn-{T}eller
{T}ransition in {C}o{T}i 2 {O} 5},
journal = {Physical review letters},
volume = {134},
number = {25},
issn = {0031-9007},
address = {College Park, Md.},
publisher = {APS},
reportid = {FZJ-2025-03550},
pages = {256702},
year = {2025},
abstract = {CoTi2O5has the paradox that low temperature static
magnetic order is incompatible with the crystal structure
owing to a mirror plane that exactly frustrates magnetic
interactions. Despite no observable structural distortion
with diffraction, CoTi2O5does magnetically order below
𝑇𝑁∼25 Kwith the breaking of spin ground state
degeneracy proposed to be a realization of the spin
Jahn-Teller effect in analogy to the celebrated orbital
Jahn-Teller transition. We apply neutron and Raman
spectroscopy to study the dynamics of this transition in
CoTi2O5. We find anomalous acoustics associated with a
symmetry breaking strain that characterizes the spin
Jahn-Teller transition. Crucially, the energy of this phonon
coincides with the energy scale of the magnetic excitations,
and has the same symmetry of an optic mode, observed with
Raman spectroscopy, which atypically softens in energy with
decreasing temperature. Taken together, we propose that the
energetics of the spin Jahn-Teller effect in CoTi2O5are
related to cooperative magnetoelastic fluctuations as
opposed to conventional soft critical dynamics which
typically drive large measurable static displacements.},
cin = {JCNS-2 / JARA-FIT / JCNS-ILL},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-2-20110106 / $I:(DE-82)080009_20140620$ /
I:(DE-Juel1)JCNS-ILL-20110128},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / 6G4 - Jülich Centre for Neutron
Research (JCNS) (FZJ) (POF4-6G4)},
pid = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G4},
typ = {PUB:(DE-HGF)16},
doi = {10.1103/sr9s-ll1y},
url = {https://juser.fz-juelich.de/record/1045689},
}