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@ARTICLE{Hussain:1046743,
author = {Hussain, Mazhar and Koers, Lucas Mues genannt and Spahn,
Ingo and Spellerberg, Stefan and Neumaier, Bernd and Qaim,
Syed M.},
title = {{P}ositron emission intensity in the decay of 72{A}s for
use in {PET} studies},
journal = {Radiochimica acta},
volume = {113},
number = {8},
issn = {0033-8230},
address = {Berlin},
publisher = {De Gruyter},
reportid = {FZJ-2025-03942},
pages = {601 - 609},
year = {2025},
note = {This work was supported by the Alexander von Humboldt (AvH)
Foundation of the Federal Republic of Germany. The author M.
Hussain is very grateful to AvH for the research fellowship
and funding under its Georg Forster program for senior
researchers.},
abstract = {72As is a β+-emitter (T1/2 = 26.0 h; Eβ+ = 1.17 MeV,Iβ+
= 87.8 $\%)$ that can be produced at a cyclotron and has
significant potential for use in PET studies. Experiments
have been undertaken to determine its positron emission
intensity with greater precision. Thin enriched 72Ge targets
were irradiated with protons of energies around 9 MeV at the
cyclotron BC1710 of the Forschungszentrum Jülich. Three
different counting methods were used: high-resolution γ-ray
spectroscopy, beta counting and X-ray spectroscopy. The
major γ-ray peaks of 72As formed via the 72Ge(p,n)72As
reaction were analysed to calculate its absolute
radioactivity, while the annihilation radiation was
characterized by a careful analysis of the 511 keV peak.
Beta counting of the same samples was undertaken over a long
period of time to validate the results. X-ray counting was
also carried out to obtain the integral decay of 72As via
electron capture (EC).The measurements furnished a total
positron decay (87.3 ± 3.7 $\%)$ and total EC decay (12.7
± 0.6 $\%).$ These experimental values agree with those
deduced from a detailed evaluation of the decay scheme of
72As.},
cin = {INM-5},
ddc = {610},
cid = {I:(DE-Juel1)INM-5-20090406},
pnm = {5253 - Neuroimaging (POF4-525)},
pid = {G:(DE-HGF)POF4-5253},
typ = {PUB:(DE-HGF)16},
doi = {10.1515/ract-2025-0005},
url = {https://juser.fz-juelich.de/record/1046743},
}