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@ARTICLE{Hilger:1046984,
author = {Hilger, Martin and El Jardali, Khaled and Feyzi, Vafa and
Vakhrameev, Daniil and Naumenko, Dmitry and Schwaiger, Ruth
and Iribarren, Diego and Lenser, Christian and Guillon,
Olivier and Menzler, Norbert H.},
title = {{T}owards sustainable interconnects for solid oxide cells:
{A}n integrated technical and environmental evaluation of
coating methods},
journal = {Journal of power sources},
volume = {659},
issn = {0378-7753},
address = {New York, NY [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2025-04052},
pages = {238471 -},
year = {2025},
abstract = {This work presents a comprehensive evaluation of three
industrially relevant coating processes – atmospheric
plasma spraying (APS), wet powder spraying (WPS), and
electrophoretic deposition (EPD) – for the application of
MnCo1.9Fe0.1O4 (MCF) spinel-based protective layers on solid
oxide cell (SOC) interconnects. Using Crofer-type ferritic
stainless steels as substrate, the coatings were assessed
with respect to their technical performance and
environmental impact. Microstructural characterization,
topography analysis for relevant interconnect structures,
and mid-term exposure tests at 800 °C in air confirm that
all three methods can produce uniform, well-adhering, and
protective coatings compatible with SOC stack integration.
While APS serves as a technologically mature reference, the
suspension-based techniques WPS and EPD demonstrate
comparable protective functionality after suitable thermal
treatments. Furthermore, life cycle assessment reveals
significant sustainability benefits for the newer methods
– especially EPD – due to lower energy demand and
enhanced material efficiency. The results highlight WPS and
EPD as promising, environmentally advantageous alternatives
for large-scale application of protective interconnect
coatings in SOC systems.},
cin = {IMD-2 / IMD-1},
ddc = {620},
cid = {I:(DE-Juel1)IMD-2-20101013 / I:(DE-Juel1)IMD-1-20101013},
pnm = {1231 - Electrochemistry for Hydrogen (POF4-123) / NOUVEAU -
NOVEL ELECTRODE COATINGS AND INTERCONNECT FOR SUSTAINABLE
AND REUSABLE SOEC (101058784) / SOFC - Solid Oxide Fuel Cell
(SOFC-20140602)},
pid = {G:(DE-HGF)POF4-1231 / G:(EU-Grant)101058784 /
G:(DE-Juel1)SOFC-20140602},
typ = {PUB:(DE-HGF)16},
doi = {10.1016/j.jpowsour.2025.238471},
url = {https://juser.fz-juelich.de/record/1046984},
}