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@ARTICLE{Heuer:1047019,
      author       = {Heuer, Philip and Ketter, Lukas and Rana, Moumita and
                      Scharf, Felix and Brunklaus, Gunther and Zeier, Wolfgang},
      title        = {{A}ttaining a fast-conducting, hybrid solid state separator
                      for all solid-state batteries through a facile wet
                      infiltration method},
      journal      = {Energy advances},
      volume       = {4},
      issn         = {2753-1457},
      address      = {Beijing},
      publisher    = {Royal Society of Chemistry},
      reportid     = {FZJ-2025-04075},
      pages        = {1356-1362},
      year         = {2025},
      abstract     = {Thin, fast-conducting and mechanically robust separators
                      are expected to be advantageous in enabling all-solid-state
                      batteries with high energy densities and good
                      electrochemical performance. In this study, a potentially
                      new scalable fabrication route for flexible
                      thiophosphate–polymer separator membranes is demonstrated.
                      By infiltrating a commercially available polymer mesh with
                      the highly conductive inorganic solid ion conductor
                      $Li_{5.5}PS_{4.5}Cl_{1.5}$, a hybrid separator membrane with
                      a high ionic conductivity is realized. The electrochemical
                      evaluation via rate capability tests reveals superior
                      performance at low stack pressures and high C-rates, when
                      comparing cells employing the hybrid membrane separator, to
                      cells utilizing conventional solid electrolyte separators.
                      As a proof of concept, a full cell implementing the hybrid
                      membrane between a Si-based anode and a
                      $LiNi_{0.83}Co_{0.11}Mn_{0.06}O_2–Li_{5.5}PS_{4.5}Cl_{1.5}$
                      composite cathode is evaluated. The experimental work is
                      complemented by resistor network modelling of the hybrid
                      membrane sheets, shedding light on potential challenges in
                      cell operation.},
      cin          = {IMD-4},
      ddc          = {620},
      cid          = {I:(DE-Juel1)IMD-4-20141217},
      pnm          = {1222 - Components and Cells (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1222},
      typ          = {PUB:(DE-HGF)16},
      doi          = {10.1039/D5YA00141B},
      url          = {https://juser.fz-juelich.de/record/1047019},
}