| Hauptseite > Publikationsdatenbank > Attaining a fast-conducting, hybrid solid state separator for all solid-state batteries through a facile wet infiltration method > print |
| 001 | 1047019 | ||
| 005 | 20260109202555.0 | ||
| 024 | 7 | _ | |a 10.1039/D5YA00141B |2 doi |
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| 037 | _ | _ | |a FZJ-2025-04075 |
| 082 | _ | _ | |a 620 |
| 100 | 1 | _ | |a Heuer, Philip |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a Attaining a fast-conducting, hybrid solid state separator for all solid-state batteries through a facile wet infiltration method |
| 260 | _ | _ | |a Beijing |c 2025 |b Royal Society of Chemistry |
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| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 520 | _ | _ | |a Thin, fast-conducting and mechanically robust separators are expected to be advantageous in enabling all-solid-state batteries with high energy densities and good electrochemical performance. In this study, a potentially new scalable fabrication route for flexible thiophosphate–polymer separator membranes is demonstrated. By infiltrating a commercially available polymer mesh with the highly conductive inorganic solid ion conductor $Li_{5.5}PS_{4.5}Cl_{1.5}$, a hybrid separator membrane with a high ionic conductivity is realized. The electrochemical evaluation via rate capability tests reveals superior performance at low stack pressures and high C-rates, when comparing cells employing the hybrid membrane separator, to cells utilizing conventional solid electrolyte separators. As a proof of concept, a full cell implementing the hybrid membrane between a Si-based anode and a $LiNi_{0.83}Co_{0.11}Mn_{0.06}O_2–Li_{5.5}PS_{4.5}Cl_{1.5}$ composite cathode is evaluated. The experimental work is complemented by resistor network modelling of the hybrid membrane sheets, shedding light on potential challenges in cell operation. |
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| 700 | 1 | _ | |a Ketter, Lukas |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Rana, Moumita |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Scharf, Felix |0 P:(DE-Juel1)188525 |b 3 |
| 700 | 1 | _ | |a Brunklaus, Gunther |0 P:(DE-Juel1)172047 |b 4 |
| 700 | 1 | _ | |a Zeier, Wolfgang |0 P:(DE-Juel1)184735 |b 5 |e Corresponding author |
| 773 | _ | _ | |a 10.1039/D5YA00141B |g p. 10.1039.D5YA00141B |0 PERI:(DE-600)3168416-6 |p 1356-1362 |t Energy advances |v 4 |y 2025 |x 2753-1457 |
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