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@ARTICLE{Fu:1048140,
author = {Fu, Chun-Yu and Kohl, Joshua B. and Liebsch, Filip and
D’Andrea, Davide and Ditrói, Tamás and Ogata, Seiryo and
Neuser, Franziska and Mai, Max and Mellis, Anna T. and
Kouroussis, Emilia and Morita, Masanobu and Gehling, Titus
and Santamaria-Araujo, José Angel and Yeo, Sin Yuin and
Endepols, Heike and Křížková, Michaela and Kozich,
Viktor and Krueger, Marcus and Hennermann, Julia B. and
Barayeu, Uladzimir and Akaike, Takaaki and Nagy, Peter and
Filipovic, Milos and Schwarz, Guenter},
title = {{S}ulfite oxidase deficiency causes persulfidation loss and
hydrogen sulfide release},
journal = {The journal of clinical investigation},
volume = {135},
number = {21},
issn = {0021-9738},
address = {Ann Arbor, Mich.},
publisher = {ASCJ},
reportid = {FZJ-2025-04520},
pages = {e181299},
year = {2025},
abstract = {Sulfite oxidase (SOX) deficiency is a rare inborn error of
cysteine metabolism resulting in severe neurological damage.
In patients, sulfite accumulates to toxic levels, causing a
rise in the downstream products S-sulfocysteine, which
mediates excitotoxicity, and thiosulfate, a catabolic
intermediate/product of hydrogen sulfide (H2S) metabolism.
Here, we report a full-body knockout mouse model for SOX
deficiency (SOXD) with a severely impaired phenotype. Among
the urinary biomarkers, thiosulfate showed a 45-fold
accumulation in SOXD mice, representing the major excreted
S-metabolite. Consistently, we found increased plasma H2S,
which was derived from sulfite-induced release from
persulfides, as demonstrated in vitro and in vivo. Mass
spectrometry analysis of total protein persulfidome
identified a major loss of S-persulfidation in $20\%$ of the
proteome, affecting enzymes in amino acids, fatty acid
metabolism, and cytosolic iron-sulfur cluster biogenesis.
Urinary amino acid profiles indicated metabolic rewiring and
mitochondrial dysfunction, thus identifying an altered H2S
metabolism and persulfidation in SOXD. Finally, oxidized
glutathione and glutathione trisulfide were able to scavenge
sulfite in vitro and in vivo, extending the lifespan of SOXD
mice and providing a mechanistic concept of sulfite
scavenging for the treatment of this severe metabolic
disorder of cysteine catabolism.},
cin = {INM-5},
ddc = {610},
cid = {I:(DE-Juel1)INM-5-20090406},
pnm = {5253 - Neuroimaging (POF4-525)},
pid = {G:(DE-HGF)POF4-5253},
typ = {PUB:(DE-HGF)16},
doi = {10.1172/JCI181299},
url = {https://juser.fz-juelich.de/record/1048140},
}