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@INPROCEEDINGS{Heinze:1048338,
author = {Heinze, Leonie and Kotte, T. and Rausch, R. and Demuer, A.
and Luther, S. and Feyerherm, R. and Ammerlaan, A. A. L. N.
and Zeitler, U. and Gorbunov, D. I. and Uhlarz, M. and Rule,
K. C. and Wolter, A. U. B. and Kühne, H. and Wosnitza, J.
and Karrasch, C. and Süllow, S.},
title = {{Q}uantum criticality and dimensional reduction in the
frustrated sawtooth chain compound atacamite},
reportid = {FZJ-2025-04560},
year = {2025},
abstract = {We present evidence for the presence of a field-induced
quantum critical point (QCP) at 21.9(1) T (H || c axis) in
the frustrated quantum magnet atacamite Cu$_2$Cl(OH)$_3$, a
mineral which we have recently identified as a material
realization of sawtooth chains [J ~ 336 K (basal-basal), J'
~ 102 K (basal-apical)]. Residual interchain couplings lead
to long-range antiferromagnetic order in atacamite below
$T_\mathrm{N}$ = 8.9(1) K. Through extensive high-field
studies of the heat capacity, we were able to map the
entropy landscape of atacamite up to 35 T. It features
highly distorted isentropes indicative of quantum
criticality in the material. By further combining
macroscopic and microscopic high-field measurement
techniques, we provide evidence for the QCP at 21.9(1) T to
separate field regions with and without long-range magnetic
order, but far away from full polarization of the material.
Underpinned by numerical results we propose this behavior to
be relatedto an effective dimensional reduction of the
material, where the chains decouple into independent
subunits. We interpret this behavior as a special type of
dimensional reduction caused by the interchain network.},
month = {May},
date = {2025-05-25},
organization = {International Conference on Highly
Frustrated Magnetism, Toronto (Canada),
25 May 2025 - 30 May 2025},
subtyp = {After Call},
cin = {JCNS-4 / JCNS-3 / MLZ / JCNS-FRM-II},
cid = {I:(DE-Juel1)JCNS-4-20201012 / I:(DE-Juel1)JCNS-3-20170926 /
I:(DE-588b)4597118-3 / I:(DE-Juel1)JCNS-FRM-II-20110218},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (FZJ)
(POF4-6G4) / 632 - Materials – Quantum, Complex and
Functional Materials (POF4-632)},
pid = {G:(DE-HGF)POF4-6G4 / G:(DE-HGF)POF4-632},
experiment = {EXP:(DE-MLZ)NOSPEC-20140101},
typ = {PUB:(DE-HGF)6},
url = {https://juser.fz-juelich.de/record/1048338},
}