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@ARTICLE{Keppens:1048411,
author = {Keppens, Arno and Hubert, Daan and Granville, José and
Nath, Oindrila and Lambert, Jean-Christopher and Wespes,
Catherine and Coheur, Pierre-François and Clerbaux, Cathy
and Boynard, Anne and Siddans, Richard and Latter, Barry and
Kerridge, Brian and Di Pede, Serena and Veefkind, Pepijn and
Cuesta, Juan and Dufour, Gaelle and Heue, Klaus-Peter and
Coldewey-Egbers, Melanie and Loyola, Diego and
Orfanoz-Cheuquelaf, Andrea and Maratt Satheesan, Swathi and
Eichmann, Kai-Uwe and Rozanov, Alexei and Sofieva, Viktoria
F. and Ziemke, Jerald R. and Inness, Antje and Van Malderen,
Roeland and Hoffmann, Lars},
title = {{H}armonisation of sixteen tropospheric ozone satellite
data records},
journal = {Atmospheric measurement techniques},
volume = {18},
number = {22},
issn = {1867-1381},
address = {Katlenburg-Lindau},
publisher = {Copernicus},
reportid = {FZJ-2025-04622},
pages = {6893 - 6916},
year = {2025},
abstract = {The first Tropospheric Ozone Assessment Report (TOAR,
2014–2019) encountered several observational challenges
that limited the confidence in estimates of the burden,
short-term variability, and long-term changes of ozone in
the free troposphere. One of these challenges is the
difficulty to interpret the consistency of satellite
measurements obtained with different techniques from
multiple sensors, leading to differences in spatiotemporal
sampling, vertical smoothing, a-priori information, and
uncertainty characterisation. This motivated the Committee
on Earth Observation Satellites (CEOS) to initiate a
coordinated activity VC-20-01 on improving the assessment
and harmonisation of tropospheric ozone measured from space.
Here, we report on work that contributes to this CEOS
activity, as well as to the ongoing second TOAR assessment
(TOAR-II, 2020–2025). Our objective is to harmonise the
spatiotemporal perspective of (sixteen) satellite ozone data
records, thereby accounting as much as possible for
differences in vertical smoothing and sampling. Four
harmonisation methods are presented to achieve this goal:
two for ozone profiles obtained from nadir sounders
(UV-visible, IR, and combined UV-IR), and two for
tropospheric ozone column products derived by one of the
residual methods (Convective Cloud Differential or
Limb–Nadir Matching). We discuss to what extent
harmonisation may affect assessments of the spatial
distribution, seasonal cycle, and long-term changes in free
tropospheric ozone, and we anchor the harmonised profile
data to ozonesonde measurements recently homogenised as part
of TOAR-II. We find that approaches that use global ozone
fields as a transfer standard (here the Copernicus
Atmosphere Monitoring Service ReAnalysis, CAMSRA) to
constrain the harmonisation generally lead to the largest
reduction of the inter-product dispersion (IPD) between
satellite datasets. These harmonisation efforts, however,
only partially account for the observed discrepancies
between the satellite datasets, with a reduction of about
$10 \%–40 \%$ of the IPD upon harmonisation, depending
on the products involved and with strong spatiotemporal
dependences. This work therefore provides evidence that it
is not only the differences in spatiotemporal smoothing and
sampling, but rather the differences in measurement
uncertainty that pose the main challenge to the assessment
of the spatial distribution and temporal evolution of free
tropospheric ozone from satellite observations.},
cin = {JSC},
ddc = {550},
cid = {I:(DE-Juel1)JSC-20090406},
pnm = {5111 - Domain-Specific Simulation $\&$ Data Life Cycle Labs
(SDLs) and Research Groups (POF4-511)},
pid = {G:(DE-HGF)POF4-5111},
typ = {PUB:(DE-HGF)16},
doi = {10.5194/amt-18-6893-2025},
url = {https://juser.fz-juelich.de/record/1048411},
}