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@PHDTHESIS{Cuma:1048441,
author = {Cuma, David},
othercontributors = {Voigtländer, Bert and Morgenstern, Markus},
title = {{M}ulti-tip scanning tunneling potentiometry on thin
bismuth films and topological insulators in a cryogenic
system},
school = {RWTH Aachen},
type = {Dissertation},
publisher = {RWTH Aachen University},
reportid = {FZJ-2025-04647},
pages = {pages 1 Online-Ressource : Illustrationen, Diagramme},
year = {2023},
note = {Dissertation, RWTH Aachen, 2023},
abstract = {A multi-tip scanning tunneling microscope (STM) is a great
tool to investigate charge transport properties of
nanostructured surfaces. This work focuses on the
utilization of multi-tip STM implemented scanning tunneling
potentiometry (STP) measurements, which allow for the
simultaneous acquisition of topography and potential
information of the sample under investigation. A detailed
insight into the measurement principles and setup as well as
theoretical considerations on this measurement method is
given in chapter 2. With the means of STP at hand, chapter 3
makes charge transport around nanoscale defects in thin
bismuth{012} films, which crystallize in a black phosphorus
like structure, the subject of discussion. Potential maps
recorded around those defects reveal the formation of
transport dipoles, which exhibit different characteristics
depending on the underlying transport regime. Comparing the
measurement data with numerical calculations and resistor
network simulations gives indications for the transition
from classical to quantum mechanical charge transport in
real space. The results presented in this chapter motivate
the need for a new STP setup at cryogenic temperatures,
which is introduced in chapter 4. The chapter reports a new
four-tip STM seated in a static bath cryostat combined with
a scanning electron microscope (SEM) used to monitor the tip
movements. Additionally, the STM's and SEM's performance
properties are characterized and the ultra-high vacuum
chamber and cryostat as well as the vibration isolation
system are described. Chapter 5 presents potentiometry
measurements in the cryogenic setup. The first part of the
chapter discusses thermo voltage signals in thin Bi(001) lms
crystallizing in a hexagonal structure. Those measurements
illustrate the existence of edge states depending on the
step edge type. Furthermore, a performance benchmark for STP
measurements in the setup is established. The second part of
the chapter characterizes the temperature dependence of
one-dimensional crystal defects and step edges in the
ternary topological insulator system (Bi1-xSbx)2Te3. It
demonstrates a decreased line defect conductivity at lower
temperatures, seemingly contradicting an increased
suppression of backscattering in topological surface states.
A suppressed backscattering can be expected at low
temperatures due to less multi-scattering events at crystal
defects.},
cin = {PGI-3},
ddc = {530},
cid = {I:(DE-Juel1)PGI-3-20110106},
pnm = {5213 - Quantum Nanoscience (POF4-521)},
pid = {G:(DE-HGF)POF4-5213},
typ = {PUB:(DE-HGF)11},
doi = {10.18154/RWTH-2023-07800},
url = {https://juser.fz-juelich.de/record/1048441},
}