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@INPROCEEDINGS{Bartoli:1050251,
author = {Bartoli, Francesco and salavei, andrei and Hilche, Tobias
and Kiran, Kiran and Fröhlich, Kristina and Treutlein,
Leander and Wolf, Niklas and Mehlkoph, Tobias and Karl,
André and Jodat, Eva and Eichel, Rüdiger-A.},
title = {{O}ptimization of {B}lade {C}oating {P}rocesses for the
{P}roduction of {L}arge {S}cale {PEMEC} {MEA}s with {L}ow
{I}ridium {L}oading},
reportid = {FZJ-2026-00063},
year = {2025},
abstract = {Current efforts in the development of Proton Exchange
Membrane Water Electrolysis (PEMWE) are driven by the
ongoing energy transition and the need to phase out fossil
fuels, to reduce dependence on other countries for energy
supply. However, since this technology strongly relies on
precious metals for their functioning, it is imperative to
reduce their content while ensuring good performances.
Stability overtime is also a major concern, since these
devices are expected to operate for hundreds of hours while
delivering the same amount of H2 throughout their life
cycle.In this work we present our recent results regarding
the preparation of Membrane Electrode Assemblies (MEAs) made
with supported catalyst commercially available and their
performance on PEMWE.Firstly, we prepared the ink containing
the catalyst powder (Pt/C for the cathode and IrOx/TiOx for
the anode), DI water, IPA and Nafion ionomer. The mixtures
were ultrasonicated and the resulting slurries were used for
the deposition process on Kapton HN substrates by Doctor
Blade technique. This technique was chosen since it is
easily transferable to roll-to-roll compatible slot-die
coating, and hence for industrial application. Through decal
transfer process, catalyst layers of 25 cm2 were transferred
on Nafion 115 using a hot press machine, the MEA was named
Ir75OxTiOx|N115|PtC. Pt and Ir loading of cathode and anode
were 0.22 and 0.35 mg/cm2 respectively. Scanning electron
microscopy (SEM) was used to study the MEAs´ morphology and
cross section. In order to record stable results under
realistic conditions, the cell was subjected to 50 hours of
conditioning, in which the current density was increased
stepwise from 0.5, 1.0, 1.5 and finally 2.0 A/cm2. Then a
polarization curve was recorded, here performance of
Ir75OxTiOx|N115|PtC was reported; the plot show how at 1.0
A/cm2 the cell voltage was only 1.8 V, a very low value
considering that the Ir load was only 0.35 mg/cm2. Stability
curve at 2.0 A/cm2 was recorded after 50 h of conditioning,
showing no sign of degradation, paving the way for future
scale-up further to 100 cm2 and beyond.},
month = {Sep},
date = {2025-09-07},
organization = {76th Annual ISE Meeting Mainz, Mainz
(Germany), 7 Sep 2025 - 12 Sep 2025},
subtyp = {After Call},
cin = {IET-1},
cid = {I:(DE-Juel1)IET-1-20110218},
pnm = {1231 - Electrochemistry for Hydrogen (POF4-123)},
pid = {G:(DE-HGF)POF4-1231},
typ = {PUB:(DE-HGF)6},
url = {https://juser.fz-juelich.de/record/1050251},
}