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@ARTICLE{Leidl:1050257,
author = {Leidl, Max Leo and Sturm, Sebastian and Filopoulou,
Aikaterina and Sachse, Carsten and Müller-Caspary, Knut},
title = {{T}owards a {P}rotein-{S}ize {D}ependent {R}esolution
{L}imit due to {D}ynamical {S}cattering in
{C}ryo-transmission {E}lectron {M}icroscopy},
journal = {Microscopy and microanalysis},
volume = {31},
number = {6},
issn = {1079-8501},
address = {Oxford},
publisher = {Oxford University Press},
reportid = {FZJ-2026-00069},
pages = {ozaf123},
year = {2025},
abstract = {In cryo-transmission electron microscopy, single-particle
reconstructions exploit the weak phase object approximation.
A decisive aspect to be studied systematically is to what
extent underlying scattering assumptions limit the
resolution, whether theoretical limits are compatible with
experimental observations, and if current experimental
benchmarks achieve this limit. Single-, multislice, and
hybrid scattering models are employed in this work for
simulating eight protein complexes up to 97.5 nm in
thickness, embedded in low-density amorphous ice obtained
from molecular dynamics. With the multislice scheme
providing an accurate solution to the multiple scattering
problem as reference, the reliability of the different
models is assessed in both real and Fourier space,
particularly via Fourier ring correlations at the specimen
exit wave level. A comparison with benchmarking literature
resolutions is performed. Our results show proportionality
of the attainable resolution to the square root of the
projection thickness. This is in reasonable quantitative
agreement with the highest resolution published
experimentally for proteins with at least the size of
apoferritin. The study provides a rationale for the
expectable resolution for a protein complex of known size.
The implications of structural noise due to the ice
background for the minimal ice thickness on protein
size-dependent resolution are discussed, as well as
efficient methods to approximate multiple scattering and
propagation in thick proteins.},
cin = {ER-C-3},
ddc = {500},
cid = {I:(DE-Juel1)ER-C-3-20170113},
pnm = {5352 - Understanding the Functionality of Soft Matter and
Biomolecular Systems (POF4-535) / 5241 - Molecular
Information Processing in Cellular Systems (POF4-524) /
4D-BioSTEM (DE002325)},
pid = {G:(DE-HGF)POF4-5352 / G:(DE-HGF)POF4-5241 /
G:(DE-Juel-1)DE002325},
typ = {PUB:(DE-HGF)16},
doi = {10.1093/mam/ozaf123},
url = {https://juser.fz-juelich.de/record/1050257},
}