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001050503 1001_ $$0P:(DE-HGF)0$$aPark, Geon-Tae$$b0
001050503 245__ $$aZero-strain Mn-rich layered cathode for sustainable and high-energy next-generation batteries
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001050503 520__ $$aThe increasing demand for high-energy Li-ion batteries for theelectrification of personal transportation may lead to uncertainty inthe global supply of raw materials (Co and Ni). Here we propose a novelMn-rich composition, which has a quasi-ordered structure with previouslyunobserved two intermixed cation-ordering sequences. The partiallyordered structure stabilizes the delithiated cathode at a high cut-off voltage,offering strain-free characteristics, with structural variations along boththe a and c axes limited to approximately 1%. Consequently, the cathode canoperate at 4.6 V while delivering a reversible capacity comparable to that ofNi-rich Li(Ni0.8Co 0.1Mn0.1)O2. Moreover, a high capacity is maintained duringlong-term and high-voltage cycling in full cells with exceptional thermalsafety. The high-performance Mn-rich layered cathodes characterized byquasi-ordered crystal structure can potentially relieve supply uncertaintyresulting from the rising demand for Ni in the battery industry andenvironmental concerns associated with the extraction of Ni from its ores.
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001050503 7001_ $$0P:(DE-HGF)0$$aPark, Nam-Yung$$b1
001050503 7001_ $$0P:(DE-HGF)0$$aRyu, Ji-Hyun$$b2
001050503 7001_ $$0P:(DE-HGF)0$$aSohn, Sung-June$$b3
001050503 7001_ $$0P:(DE-HGF)0$$aYu, Tae-Yeon$$b4
001050503 7001_ $$0P:(DE-HGF)0$$aKim, Myoung-Chan$$b5
001050503 7001_ $$0P:(DE-Juel1)196973$$aBaiju, Sourav$$b6$$ufzj
001050503 7001_ $$0P:(DE-Juel1)174502$$aKaghazchi, Payam$$b7
001050503 7001_ $$0P:(DE-HGF)0$$aYoon, Chong S.$$b8$$eCorresponding author
001050503 7001_ $$0P:(DE-HGF)0$$aSun, Yang-Kook$$b9$$eCorresponding author
001050503 773__ $$0PERI:(DE-600)2847369-3$$a10.1038/s41560-025-01852-3$$gVol. 10, no. 10, p. 1215 - 1225$$n10$$p1215 - 1225$$tNature energy$$v10$$x2058-7546$$y2025
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