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@ARTICLE{Park:1050503,
      author       = {Park, Geon-Tae and Park, Nam-Yung and Ryu, Ji-Hyun and
                      Sohn, Sung-June and Yu, Tae-Yeon and Kim, Myoung-Chan and
                      Baiju, Sourav and Kaghazchi, Payam and Yoon, Chong S. and
                      Sun, Yang-Kook},
      title        = {{Z}ero-strain {M}n-rich layered cathode for sustainable and
                      high-energy next-generation batteries},
      journal      = {Nature energy},
      volume       = {10},
      number       = {10},
      issn         = {2058-7546},
      address      = {London},
      publisher    = {Nature Publishing Group},
      reportid     = {FZJ-2026-00271},
      pages        = {1215 - 1225},
      year         = {2025},
      abstract     = {The increasing demand for high-energy Li-ion batteries for
                      theelectrification of personal transportation may lead to
                      uncertainty inthe global supply of raw materials (Co and
                      Ni). Here we propose a novelMn-rich composition, which has a
                      quasi-ordered structure with previouslyunobserved two
                      intermixed cation-ordering sequences. The partiallyordered
                      structure stabilizes the delithiated cathode at a high
                      cut-off voltage,offering strain-free characteristics, with
                      structural variations along boththe a and c axes limited to
                      approximately $1\%.$ Consequently, the cathode canoperate at
                      4.6 V while delivering a reversible capacity comparable to
                      that ofNi-rich Li(Ni0.8Co 0.1Mn0.1)O2. Moreover, a high
                      capacity is maintained duringlong-term and high-voltage
                      cycling in full cells with exceptional thermalsafety. The
                      high-performance Mn-rich layered cathodes characterized
                      byquasi-ordered crystal structure can potentially relieve
                      supply uncertaintyresulting from the rising demand for Ni in
                      the battery industry andenvironmental concerns associated
                      with the extraction of Ni from its ores.},
      cin          = {IMD-2},
      ddc          = {330},
      cid          = {I:(DE-Juel1)IMD-2-20101013},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      doi          = {10.1038/s41560-025-01852-3},
      url          = {https://juser.fz-juelich.de/record/1050503},
}