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| 001 | 1050503 | ||
| 005 | 20260116204418.0 | ||
| 024 | 7 | _ | |a 10.1038/s41560-025-01852-3 |2 doi |
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| 100 | 1 | _ | |a Park, Geon-Tae |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a Zero-strain Mn-rich layered cathode for sustainable and high-energy next-generation batteries |
| 260 | _ | _ | |a London |c 2025 |b Nature Publishing Group |
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| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 520 | _ | _ | |a The increasing demand for high-energy Li-ion batteries for theelectrification of personal transportation may lead to uncertainty inthe global supply of raw materials (Co and Ni). Here we propose a novelMn-rich composition, which has a quasi-ordered structure with previouslyunobserved two intermixed cation-ordering sequences. The partiallyordered structure stabilizes the delithiated cathode at a high cut-off voltage,offering strain-free characteristics, with structural variations along boththe a and c axes limited to approximately 1%. Consequently, the cathode canoperate at 4.6 V while delivering a reversible capacity comparable to that ofNi-rich Li(Ni0.8Co 0.1Mn0.1)O2. Moreover, a high capacity is maintained duringlong-term and high-voltage cycling in full cells with exceptional thermalsafety. The high-performance Mn-rich layered cathodes characterized byquasi-ordered crystal structure can potentially relieve supply uncertaintyresulting from the rising demand for Ni in the battery industry andenvironmental concerns associated with the extraction of Ni from its ores. |
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| 700 | 1 | _ | |a Park, Nam-Yung |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Ryu, Ji-Hyun |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Sohn, Sung-June |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Yu, Tae-Yeon |0 P:(DE-HGF)0 |b 4 |
| 700 | 1 | _ | |a Kim, Myoung-Chan |0 P:(DE-HGF)0 |b 5 |
| 700 | 1 | _ | |a Baiju, Sourav |0 P:(DE-Juel1)196973 |b 6 |u fzj |
| 700 | 1 | _ | |a Kaghazchi, Payam |0 P:(DE-Juel1)174502 |b 7 |
| 700 | 1 | _ | |a Yoon, Chong S. |0 P:(DE-HGF)0 |b 8 |e Corresponding author |
| 700 | 1 | _ | |a Sun, Yang-Kook |0 P:(DE-HGF)0 |b 9 |e Corresponding author |
| 773 | _ | _ | |a 10.1038/s41560-025-01852-3 |g Vol. 10, no. 10, p. 1215 - 1225 |0 PERI:(DE-600)2847369-3 |n 10 |p 1215 - 1225 |t Nature energy |v 10 |y 2025 |x 2058-7546 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/1050503/files/s41560-025-01852-3.pdf |y OpenAccess |
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