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@ARTICLE{Bertram:1052066,
      author       = {Bertram, Franziska and Hofmann, Jörg and Gottschalk, Jan
                      and Weißenberg, Felix and Brands, Thorsten and Holly, Carlo
                      and Jupke, Andreas},
      title        = {{D}evelopment of a two-dimensional {R}aman spectroscopy
                      measuring technique for the visualization of mass transfer
                      during droplet formation},
      journal      = {Chemical engineering science},
      volume       = {320},
      issn         = {0009-2509},
      address      = {Amsterdam [u.a.]},
      publisher    = {Elsevier Science},
      reportid     = {FZJ-2026-00736},
      pages        = {122444 -},
      year         = {2026},
      abstract     = {A novel two-dimensional Raman spectroscopy measurement
                      setup is developed to visualize mass transfer during droplet
                      formation and applied to the water/acetonitrile/toluene
                      system. This setup enables direct observation of local
                      solute contents. Experiments were conducted using 2 mm and 4
                      mm droplets with an initial acetonitrile content of 10
                      $wt\%.$ The results are qualitatively consistent with
                      findings reported in the literature for similar systems.
                      Initial calibration measurements using single-phase systems
                      demonstrated linear correlations between measured
                      intensities and solute contents in both phases, though a
                      baseline shift in the organic phase was attributed to the
                      presence of toluene. Applying these correlations to droplet
                      formation experiments resulted in an overestimation of local
                      acetonitrile contents. Future work will focus on further
                      refining the quantification capabilities of the measurement
                      setup.},
      cin          = {IBG-2},
      ddc          = {660},
      cid          = {I:(DE-Juel1)IBG-2-20101118},
      pnm          = {2172 - Utilization of renewable carbon and energy sources
                      and engineering of ecosystem functions (POF4-217) / PFExC006
                      - EXC2186 "The Fuel Science Center" (EXS-PF-PFExC006)},
      pid          = {G:(DE-HGF)POF4-2172 / G:(DE-82)EXS-PF-PFExC006},
      typ          = {PUB:(DE-HGF)16},
      doi          = {10.1016/j.ces.2025.122444},
      url          = {https://juser.fz-juelich.de/record/1052066},
}