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@ARTICLE{Nicolai:1052236,
author = {Nicolai, Hendrik and Schuh, Vinzenz and Bähr, Antonia and
Schneider, Max and Rong, Felix and Kaddar, Driss and Bode,
Mathis and Hasse, Christian},
title = {{L}aminar and turbulent hydrogen-enriched methane flames:
{I}nteraction of thermodiffusive instabilities and local
fuel demixing},
journal = {Proceedings of the Combustion Institute},
volume = {41},
issn = {1540-7489},
address = {Amsterdam [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2026-00855},
pages = {105885},
year = {2025},
abstract = {Blending hydrogen with methane provides a practical
approach for transitioning existing energy infrastructure to
hydrogen-based carriers. However, under fuel-lean
conditions, increasing the hydrogen content causes flames to
transition rapidly from methane-like combustion to
hydrogen-dominated flames, primarily driven by
thermodiffusive instabilities that significantly enhance
turbulent flame speeds. This study systematically examines
lean methane/hydrogen/air flames of varying complexity, from
three-dimensional laminar unstable cases to turbulent jet
flames at two different Reynolds numbers, with an emphasis
on the impact of the distinct molecular transport properties
of hydrogen and methane. The large-scale simulations reveal
that these blends exhibit instabilities even under turbulent
conditions, albeit to a lesser degree than pure hydrogen
flames. Nonetheless, synergistic interactions between
turbulence and thermodiffusive instabilities lead to notable
increases in turbulent flame speed and reactivity factors
($I_0$) at higher Reynolds/Karlovitz numbers. Moreover,
beyond the effects of overall non-unity Lewis number, the
different diffusivity of hydrogen and methane (i.e.,
non-equal Lewis numbers) significantly influence the
formation and intensity of intrinsic flame instabilities.
These findings underscore the importance of thermodiffusive
instabilities in methane/hydrogen combustion and highlight
the need for advanced modeling approaches capable of
capturing local demixing effects under turbulent flows
conditions.},
cin = {JSC},
ddc = {660},
cid = {I:(DE-Juel1)JSC-20090406},
pnm = {5112 - Cross-Domain Algorithms, Tools, Methods Labs (ATMLs)
and Research Groups (POF4-511) / Inno4Scale - Innovative
Algorithms for Applications on European Exascale
Supercomputers (101118139)},
pid = {G:(DE-HGF)POF4-5112 / G:(EU-Grant)101118139},
typ = {PUB:(DE-HGF)16},
doi = {10.1016/j.proci.2025.105885},
url = {https://juser.fz-juelich.de/record/1052236},
}