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001052276 1001_ $$00000-0002-3005-5788$$aQiu, Shudi$$b0
001052276 245__ $$aOver one-micron-thick void-free perovskite layers enable highly efficient and fully printed solar cells
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001052276 520__ $$aCommercialization of perovskite photovoltaics hinges on the successful transition from laboratory-scale fabrication to industrial-scale manufacturing. A key challenge in fully printed perovskite solar cells with non-reflecting back electrodes is the deposition of high-quality, over-one-micron-thick perovskite layers to minimize photocurrent losses from incomplete light absorption. However, the formation of voids at the substrate/perovskite interface impedes the fabrication of such layers. Here, phase-field simulations reveal that the bottom voids originate from trapped residual solvents, driven by nanocrystal aggregation at the liquid–vapor interface during drying. Guided by these insights, we introduce a two-dimensional (2D) perovskite layer-assisted growth strategy to promote heterogeneous nucleation at the substrate, accelerating 3D perovskite crystallization and preventing solvent entrapment. This strategy enables the formation of highly crystalline, monolithic perovskite films exceeding one micrometer in thickness. The resulting void-free films maximize photocurrent extraction, achieving power conversion efficiencies of 19.9% on rigid substrates and 17.5% on flexible substrates in fully printed perovskite solar cells with non-reflecting carbon electrodes.
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001052276 536__ $$0G:(GEPRIS)506698391$$aDFG project G:(GEPRIS)506698391 - Experimentelle und theoretische Untersuchungen von Prozessparametern zur Herstellung dicker und defektfreier Perowskit-Schichten (506698391)$$c506698391$$x1
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001052276 7001_ $$0P:(DE-Juel1)187003$$aMajewski, Martin$$b1
001052276 7001_ $$00000-0002-6018-5946$$aDong, Lirong$$b2
001052276 7001_ $$00000-0003-3500-2180$$aDistler, Andreas$$b3
001052276 7001_ $$00000-0002-8399-4244$$aLi, Chaohui$$b4
001052276 7001_ $$0P:(DE-Juel1)178784$$aForberich, Karen$$b5$$ufzj
001052276 7001_ $$00000-0003-2405-4268$$aTian, Jingjing$$b6
001052276 7001_ $$00000-0002-5450-3215$$aHemasiri, Naveen Harindu$$b7
001052276 7001_ $$0P:(DE-Juel1)201377$$aLiu, Chao$$b8
001052276 7001_ $$0P:(DE-Juel1)194716$$aZhang, Jiyun$$b9
001052276 7001_ $$0P:(DE-HGF)0$$aYang, Fu$$b10
001052276 7001_ $$0P:(DE-Juel1)201923$$aLe Corre, Vincent M.$$b11
001052276 7001_ $$0P:(DE-Juel1)203175$$aBibrack, Max$$b12$$ufzj
001052276 7001_ $$00000-0002-5577-2716$$aBasu, Robin$$b13
001052276 7001_ $$0P:(DE-Juel1)210193$$aBarabash, Anastasia$$b14$$ufzj
001052276 7001_ $$0P:(DE-Juel1)167472$$aHarting, Jens$$b15
001052276 7001_ $$0P:(DE-Juel1)173965$$aRonsin, Olivier J. J.$$b16$$eCorresponding author
001052276 7001_ $$0P:(DE-Juel1)200304$$aDu, Tian$$b17
001052276 7001_ $$0P:(DE-Juel1)190193$$aEgelhaaf, Hans-Joachim$$b18
001052276 7001_ $$0P:(DE-Juel1)176427$$aBrabec, Christoph J.$$b19$$eCorresponding author
001052276 773__ $$0PERI:(DE-600)2439879-2$$a10.1039/D5EE01722J$$gVol. 18, no. 12, p. 5926 - 5939$$n12$$p5926 - 5939$$tEnergy & environmental science$$v18$$x1754-5692$$y2025
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