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@ARTICLE{Ibach:10597,
author = {Ibach, H. and Beltramo, G. L. and Giesen, M.},
title = {{I}nterface capacitance of nano-patterned electrodes},
journal = {Surface science},
volume = {605},
issn = {0039-6028},
address = {Amsterdam},
publisher = {Elsevier},
reportid = {PreJuSER-10597},
year = {2011},
note = {Record converted from VDB: 12.11.2012},
abstract = {By employing numerical solutions of the Poisson-Boltzmann
equation we have studied the interface capacitance of flat
electrodes with stripes of different potentials of zero
charge phi(pzc). The results depend on the ratio of the
width of the stripes l to the dielectric screening length in
the electrolyte, the Debye length d(Debye), as well as on
the difference Delta phi(pzc), in relation k(B)T/e. As
expected, the capacitance of a striped surface has its
minimum at the mean potential of the surface if l/d(Debye)<<
1 and displays two minima if l/d(Debye)>> 1. An unexpected
result is that for Delta phi(pzc)congruent to 0.2V, the
transition between the two extreme cases does not occur when
l congruent to d(Debye). but rather when l>10d(Debye). As a
consequence, a single minimum in the capacitance is observed
for dilute electrolytes even for 100 nm wide stripes. The
capacitance at the minimum is however higher than for
homogeneous surfaces. Furthermore, the potential at the
minimum deviates significantly from the potential of zero
mean charge on the surface if l>3d(Debye) and Delta phi(pzc)
is larger than about 4k(B)T/e. The capacitance of stepped,
partially reconstructed Au(11n) surfaces is discussed as an
example. Consequences for Parsons-Zobel-plots of the
capacitances of inhomogeneous surfaces are likewise
discussed. (C) 2010 Elsevier B.V. All rights reserved.},
keywords = {J (WoSType)},
cin = {IBN-4},
ddc = {540},
cid = {I:(DE-Juel1)VDB802},
pnm = {BioSoft: Makromolekulare Systeme und biologische
Informationsverarbeitung},
pid = {G:(DE-Juel1)FUEK505},
shelfmark = {Chemistry, Physical / Physics, Condensed Matter},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000286021000034},
doi = {10.1016/j.susc.2010.10.025},
url = {https://juser.fz-juelich.de/record/10597},
}