TY - JOUR
AU - Atodiresei, N.
AU - Brede, J.
AU - Lazic, P.
AU - Caciuc, V.
AU - Hoffmann, G.
AU - Wiesendanger, R.
AU - Blügel, S.
TI - Design of the Local Spin Polarization at the Organic-Ferromagnetic Interface
JO - Physical review letters
VL - 105
SN - 0031-9007
CY - College Park, Md.
PB - APS
M1 - PreJuSER-10761
SP - 066601
PY - 2010
N1 - This work is funded by the DFG (SPP1243, SFB 668-A5 and GrK 611) and Alexander von Humboldt Foundation. The computations were performed on JUROPA and JUGENE supercomputers at the Julich Supercomputing Centre, Forschungszentrum Julich (Germany).
AB - By means of ab initio calculations and spin-polarized scanning tunneling microscopy experiments the creation of a complex energy dependent magnetic structure with a tailored spin-polarized interface is demonstrated. We show this novel effect by adsorbing organic molecules containing pi(p(z)) electrons onto a magnetic surface. The hybridization of the out-of-plane p(z) atomic-type orbitals with the d states of the metal leads to the inversion of the spin polarization at the organic site due to a p(z)-d Zener exchange-type mechanism. As a key result, we demonstrate the possibility to selectively and efficiently inject spin-up and spin-down electrons from a ferromagnetic-organic interface, an effect which can be exploited in future spintronic devices.
KW - J (WoSType)
LB - PUB:(DE-HGF)16
UR - <Go to ISI:>//WOS:000280580100008
DO - DOI:10.1103/PhysRevLett.105.066601
UR - https://juser.fz-juelich.de/record/10761
ER -