001     10761
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024 7 _ |2 DOI
|a 10.1103/PhysRevLett.105.066601
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024 7 _ |2 Handle
|a 2128/7247
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041 _ _ |a eng
082 _ _ |a 550
084 _ _ |2 WoS
|a Physics, Multidisciplinary
100 1 _ |0 P:(DE-Juel1)130513
|a Atodiresei, N.
|b 0
|u FZJ
245 _ _ |a Design of the Local Spin Polarization at the Organic-Ferromagnetic Interface
260 _ _ |a College Park, Md.
|b APS
|c 2010
300 _ _ |a 066601
336 7 _ |a Journal Article
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440 _ 0 |0 4925
|a Physical Review Letters
|v 105
|x 0031-9007
500 _ _ |a This work is funded by the DFG (SPP1243, SFB 668-A5 and GrK 611) and Alexander von Humboldt Foundation. The computations were performed on JUROPA and JUGENE supercomputers at the Julich Supercomputing Centre, Forschungszentrum Julich (Germany).
520 _ _ |a By means of ab initio calculations and spin-polarized scanning tunneling microscopy experiments the creation of a complex energy dependent magnetic structure with a tailored spin-polarized interface is demonstrated. We show this novel effect by adsorbing organic molecules containing pi(p(z)) electrons onto a magnetic surface. The hybridization of the out-of-plane p(z) atomic-type orbitals with the d states of the metal leads to the inversion of the spin polarization at the organic site due to a p(z)-d Zener exchange-type mechanism. As a key result, we demonstrate the possibility to selectively and efficiently inject spin-up and spin-down electrons from a ferromagnetic-organic interface, an effect which can be exploited in future spintronic devices.
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700 1 _ |0 P:(DE-HGF)0
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700 1 _ |0 P:(DE-HGF)0
|a Lazic, P.
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700 1 _ |0 P:(DE-Juel1)130583
|a Caciuc, V.
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700 1 _ |0 P:(DE-HGF)0
|a Hoffmann, G.
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700 1 _ |0 P:(DE-HGF)0
|a Wiesendanger, R.
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700 1 _ |0 P:(DE-Juel1)130548
|a Blügel, S.
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|y 2010
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