000111941 001__ 111941
000111941 005__ 20240529111656.0
000111941 0247_ $$2DOI$$a10.1016/j.jssc.2012.03.064
000111941 0247_ $$2WOS$$aWOS:000308047800012
000111941 037__ $$aPreJuSER-111941
000111941 041__ $$aeng
000111941 082__ $$a540
000111941 084__ $$2WoS$$aChemistry, Inorganic & Nuclear
000111941 084__ $$2WoS$$aChemistry, Physical
000111941 1001_ $$0P:(DE-HGF)0$$aPerlt, S.$$b0
000111941 245__ $$aMicrostructure analyses and thermoelectric properties of Ag1-xPb18Sb1+yTe20
000111941 260__ $$aOrlando, Fla.$$bAcademic Press$$c2012
000111941 300__ $$a58 - 63
000111941 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article
000111941 3367_ $$2DataCite$$aOutput Types/Journal article
000111941 3367_ $$00$$2EndNote$$aJournal Article
000111941 3367_ $$2BibTeX$$aARTICLE
000111941 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000111941 3367_ $$2DRIVER$$aarticle
000111941 440_0 $$08041$$aJournal of Solid State Chemistry$$v193$$x0022-4596$$yS1
000111941 500__ $$aThe authors would like to thank the BMBF (Contract 03X3540) for funding this study. S. Perlt thanks the Leibniz Institute of Surface Modification for financial support enabling research visits at UK facilities. Contributions by B. Schaffer and Q. Ramasse (both SuperSTEM facility Daresbury Laboratories, UK) are gratefully acknowledged. T. Hoche is endepted to Dr. P. Werner granting access to TEM facilities at MPI for Microstructure Physics in Halle.
000111941 520__ $$aThis study reports microstructural investigations of long-term annealed Ag1-xPbmSb1+yTe2+m (m=18, x=y=0, hereinafter referred to as AgPb18SbTe20) (Lead-Antimony-Silver-Tellurium, LAST-18) as well as of Ag1-xPb18Sb1+yTe20, i.e. Ag-deficient and Sb-excess LAST-18 (x not equal 0, y not equal 0), respectively. Two different length scales are explored. The micrometer scale was evaluated by SEM to analyze the volume fraction and the number of secondary phases as well as the impact of processing parameters on the homogeneity of bulk samples. For AgPb18SbTe20, site-specific FIB liftout of TEM lamellae from thermoelectrically characterized samples was accomplished to investigate the structure on the nanometer scale. High-resolution TEM and energy-filtered TEM were performed to reveal shape and size distribution of nanoprecipitates, respectively. A hypothesis concerning the structure-property relationship is set out within the frame of a gradient annealing experiment. This study is completed by results dealing with inhomogeneities on the micrometer scale of Ag1-xPb18Sb1+yTe20 and its electronic properties. (C) 2012 Elsevier Inc. All rights reserved.
000111941 536__ $$0G:(DE-Juel1)FUEK412$$2G:(DE-HGF)$$aGrundlagen für zukünftige Informationstechnologien (FUEK412)$$cFUEK412$$x0
000111941 536__ $$0G:(DE-HGF)POF2-544$$a544 - In-house Research with PNI (POF2-544)$$cPOF2-544$$fPOF II$$x1
000111941 588__ $$aDataset connected to Web of Science
000111941 65320 $$2Author$$aLAST
000111941 65320 $$2Author$$aMicrostructure analysis
000111941 65320 $$2Author$$aHRTEM
000111941 650_7 $$2WoSType$$aJ
000111941 7001_ $$0P:(DE-HGF)0$$aHöche, Th.$$b1
000111941 7001_ $$0P:(DE-HGF)0$$aDadda, J.$$b2
000111941 7001_ $$0P:(DE-HGF)0$$aMüller, E.$$b3
000111941 7001_ $$0P:(DE-Juel1)VDB90855$$aBauer Pereira, P.$$b4$$uFZJ
000111941 7001_ $$0P:(DE-Juel1)130706$$aHermann, R.$$b5$$uFZJ
000111941 7001_ $$0P:(DE-HGF)0$$aSarahan, M.$$b6
000111941 7001_ $$0P:(DE-HGF)0$$aPippel, E.$$b7
000111941 7001_ $$0P:(DE-HGF)0$$aBrydson, R.$$b8
000111941 773__ $$0PERI:(DE-600)1469806-7$$a10.1016/j.jssc.2012.03.064$$gVol. 193, p. 58 - 63$$p58 - 63$$q193<58 - 63$$tJournal of solid state chemistry$$v193$$x0022-4596$$y2012
000111941 8567_ $$uhttp://dx.doi.org/10.1016/j.jssc.2012.03.064
000111941 909CO $$ooai:juser.fz-juelich.de:111941$$pVDB
000111941 915__ $$0StatID:(DE-HGF)0010$$2StatID$$aJCR/ISI refereed
000111941 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR
000111941 915__ $$0StatID:(DE-HGF)0110$$2StatID$$aWoS$$bScience Citation Index
000111941 915__ $$0StatID:(DE-HGF)0111$$2StatID$$aWoS$$bScience Citation Index Expanded
000111941 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection
000111941 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bThomson Reuters Master Journal List
000111941 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS
000111941 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline
000111941 915__ $$0StatID:(DE-HGF)0420$$2StatID$$aNationallizenz
000111941 915__ $$0StatID:(DE-HGF)1040$$2StatID$$aDBCoverage$$bZoological Record
000111941 9141_ $$y2012
000111941 9132_ $$0G:(DE-HGF)POF3-623$$1G:(DE-HGF)POF3-620$$2G:(DE-HGF)POF3-600$$aDE-HGF$$bForschungsbereich Materie$$lIn-house research on the structure, dynamics and function of matter$$vNeutrons for Research on Condensed Matter$$x0
000111941 9131_ $$0G:(DE-HGF)POF2-544$$1G:(DE-HGF)POF2-540$$2G:(DE-HGF)POF2-500$$3G:(DE-HGF)POF2$$4G:(DE-HGF)POF$$aDE-HGF$$bStruktur der Materie$$lForschung mit Photonen, Neutronen, Ionen$$vIn-house Research with PNI$$x0
000111941 9201_ $$0I:(DE-Juel1)PGI-4-20110106$$gPGI$$kPGI-4$$lStreumethoden$$x0
000111941 9201_ $$0I:(DE-Juel1)JCNS-2-20110106$$gJCNS$$kJCNS-2$$lStreumethoden$$x1
000111941 9201_ $$0I:(DE-82)080009_20140620$$gJARA$$kJARA-FIT$$lJülich-Aachen Research Alliance - Fundamentals of Future Information Technology$$x2
000111941 970__ $$aVDB:(DE-Juel1)140576
000111941 980__ $$aVDB
000111941 980__ $$aConvertedRecord
000111941 980__ $$ajournal
000111941 980__ $$aI:(DE-Juel1)PGI-4-20110106
000111941 980__ $$aI:(DE-Juel1)JCNS-2-20110106
000111941 980__ $$aI:(DE-82)080009_20140620
000111941 980__ $$aUNRESTRICTED
000111941 981__ $$aI:(DE-Juel1)JCNS-2-20110106
000111941 981__ $$aI:(DE-Juel1)JCNS-2-20110106
000111941 981__ $$aI:(DE-Juel1)VDB881