TY - JOUR
AU - Sawka-Dobrowolska, W.
AU - Bator, G.
AU - Sobczyk, L.
AU - Grech, E.
AU - Nowicka-Scheibe, J.
AU - Pawlukojc, A.
AU - Wuttke, J.
TI - The (2:1) complex of picric acid with tetramethylpyrazine. The structure,l IR spectra and tunnel splitting of methyl groups
JO - Journal of molecular structure
VL - 975
SN - 0022-2860
CY - New York, NY [u.a.]
PB - Elsevier
M1 - PreJuSER-11791
PY - 2010
N1 - This work was supported by the Polish Ministry of Science and Higher Education (Project Register No. N N204 2497 34). This research project has been supported by the European Commission under the 7th Framework Programme through the Key Action: Strengthening the European Research Area, Research Infrastructures. Contract No. 226507 (NMI3).
AB - The crystal structure of 2:1 picric acid (PAH) with tetramethylpyrazine (TMP) was determined by using X-ray diffraction studies. Two equivalent N+-H center dot center dot center dot O- hydrogen bonds are formed with the length of 2.601 angstrom (calculated 2.640 angstrom). In the IR spectra very broad doublet at ca. 2000 and 2400 cm(-1) is observed, which can be interpreted as due to symmetric and asymmetric N+-H vibrations. In neutron backscattering two tunnel splittings are observed, in agreement with the symmetry of 2:1 assemblies. At 4 K the tunnel peaks are located at 3.17 and 4.24 mu eV. (C) 2010 Elsevier B.V. All rights reserved.
KW - J (WoSType)
LB - PUB:(DE-HGF)16
UR - <Go to ISI:>//WOS:000280028600045
DO - DOI:10.1016/j.molstruc.2010.04.041
UR - https://juser.fz-juelich.de/record/11791
ER -