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@ARTICLE{Kusmin:11979,
author = {Kusmin, A. and Gruener, S. and Henschel, A. and de Souza,
N.R. and Allgaier, J. and Richter, D. and Huber, P.},
title = {{P}olymer dynamics in nanochannels of porous silicon: {A}
neutron spin echo study},
journal = {Macromolecules},
volume = {43},
issn = {0024-9297},
address = {Washington, DC},
publisher = {Soc.},
reportid = {PreJuSER-11979},
pages = {8162 - 8169},
year = {2010},
note = {A.K. thanks O. Holderer and M. Monken-busch for the help
with getting familiar with NSE in general and J-NSE in
particular. This work has been supported by the German
Research Foundation (DFG) within the priority program SP
1164, Nano- and Microfluidies, Grant No. Hu 850/2.},
abstract = {Neutron spin echo spectra of poly(ethylene oxide) (PEO)
melts confined in porous silicon (the mean pore diameter: 13
nm) were recorded at Q = 0.05, 0.08, and 0.11 angstrom(-1)
and successfully analyzed in terms of a two-state model,
where chains adsorbed to the pore walls exhibit much slower
internal dynamics than in the bulk and their centers-of-mass
do not move, while free chains have hulk like internal
dynamics and diffuse within an infinite cylinder in the
center of the pore. The radius of this cylinder was found to
be 1.4 nm for PE:0 3 kg/mol (3k); this corresponds to the
thickness Idle adsorbed layer to be approximately equal to
the Flory radius. As opposed to PEO 10k, for which details
on the center of mass diffusion could not he discerned, for
PEO 3k the diffusion rate along the pore was found to he
smaller than that in the radial direction.},
keywords = {J (WoSType)},
cin = {IFF-5 / IFF-4 / Jülich Centre for Neutron Science JCNS
(JCNS) ; JCNS},
ddc = {540},
cid = {I:(DE-Juel1)VDB785 / I:(DE-Juel1)VDB784 /
I:(DE-Juel1)JCNS-20121112},
pnm = {BioSoft: Makromolekulare Systeme und biologische
Informationsverarbeitung / Großgeräte für die Forschung
mit Photonen, Neutronen und Ionen (PNI)},
pid = {G:(DE-Juel1)FUEK505 / G:(DE-Juel1)FUEK415},
experiment = {EXP:(DE-MLZ)J-NSE-20140101},
shelfmark = {Polymer Science},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000282478500042},
doi = {10.1021/ma1004925},
url = {https://juser.fz-juelich.de/record/11979},
}