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000012079 084__ $$2WoS$$aPhysics, Multidisciplinary
000012079 1001_ $$0P:(DE-HGF)0$$aKeeble, D.J.$$b0
000012079 245__ $$aIdentification of A- and B-site cation vacancy defects in perovskite oxide thin films
000012079 260__ $$aCollege Park, Md.$$bAPS$$c2010
000012079 300__ $$a226102
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000012079 440_0 $$04925$$aPhysical Review Letters$$v105$$x0031-9007$$y22
000012079 500__ $$aD. J. K. acknowledges European Commission Programme RII3-CT-2003-505925. We thank C. Hugenschmidt for providing the NEUPOMUC beam line. D. J. K. thanks I. Makkonen, Helsinki University of Technology, for MIKA/DOPPLER support.
000012079 520__ $$aCation vacancies on both sublattices (V-Ti, V-Sr) have been identified in homoepitaxial pulsed laser deposited SrTiO3 films using high intensity variable energy positron annihilation lifetime spectroscopy (PALS) measurements. Film nonstoichiometry was varied by varying laser fluence. PALS showed that on increasing the fluence above the Ti/Sr similar to 1 value, the concentration ratio [V-Sr]/[V-Ti] systematically increased. Reducing the fluence into the Ti-poor region below resulted in additional vacancy cluster defect formation. Vacancy concentrations greater than similar to 50 ppm were observed in all films.
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000012079 7001_ $$0P:(DE-Juel1)VDB95416$$aWicklein, S.$$b1$$uFZJ
000012079 7001_ $$0P:(DE-Juel1)VDB5464$$aDittmann, R.$$b2$$uFZJ
000012079 7001_ $$0P:(DE-HGF)0$$aRavelli, L.$$b3
000012079 7001_ $$0P:(DE-HGF)0$$aMackie, R.A.$$b4
000012079 7001_ $$0P:(DE-HGF)0$$aEgger, W.$$b5
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000012079 8567_ $$uhttp://dx.doi.org/10.1103/PhysRevLett.105.226102
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