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024 7 _ |a 10.1088/1367-2630/12/8/083044
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037 _ _ |a PreJuSER-12182
041 _ _ |a eng
082 _ _ |a 530
084 _ _ |2 WoS
|a Physics, Multidisciplinary
100 1 _ |0 P:(DE-Juel1)130647
|a Fu, Z.
|b 0
|u FZJ
245 _ _ |a An approach to the magnetic ground state of the molecular magnet {Mo72Fe30}
260 _ _ |a [Bad Honnef]
|b Dt. Physikalische Ges.
|c 2010
300 _ _ |a 083044
336 7 _ |a Journal Article
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440 _ 0 |0 8201
|a New Journal of Physics
|v 12
|x 1367-2630
500 _ _ |a Record converted from VDB: 12.11.2012
520 _ _ |a The nature of the magnetic ground state of the spin-frustrated molecular magnet {Mo72Fe30} is studied using polarized neutron scattering and specific heat methods. The magnetic scattering cross section up to 2.30 angstrom(-1) has been determined by means of diffuse neutron scattering with xyz polarization analysis at temperatures from 1.5 to 100 K. The spin correlations observed at 1.5 K agree well with the simulation based on the three-sublattice spin configuration model for {Mo72Fe30}. The specific heat of {Mo72Fe30} has been measured from 60 mK to 15 K under zero external magnetic field. The energy gaps, 0.09(1) and 0.64(1) meV, identified by the Schottky-type anomalies in the specific heat data are in reasonable agreement with the low-lying magnetic excitations predicted by the quantum rotational band model for the three-sublattice spin configuration model. Therefore, our experimental study provides strong support that the three-sublattice spin configuration model is a good approach to the magnetic ground state of {Mo72Fe30}.
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|e DNS: Diffuse scattering neutron time of flight spectrometer
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773 _ _ |0 PERI:(DE-600)1464444-7
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|y 2010
856 7 _ |u http://dx.doi.org/10.1088/1367-2630/12/8/083044
856 4 _ |u https://juser.fz-juelich.de/record/12182/files/Fu_2010_New_J._Phys._12_083044.pdf
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