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@ARTICLE{LangYona:12512,
author = {Lang-Yona, N. and Rudich, Y. and Mentel, T. F. and Bohne,
A. and Buchholz, A. and Kiendler-Scharr, A. and Kleist, E.
and Spindler, C. and Tillmann, R. and Wildt, J.},
title = {{T}he chemical and microphysical properties of secondary
organic aerosols from {H}olm {O}ak emissions},
journal = {Atmospheric chemistry and physics},
volume = {10},
issn = {1680-7316},
address = {Katlenburg-Lindau},
publisher = {EGU},
reportid = {PreJuSER-12512},
pages = {7253 - 7265},
year = {2010},
note = {We gratefully acknowledge the support by the European
Commission (IP-EUCAARI, Contract No. 036833-2, by the ESF
(INTROP) and by the Israel Science Foundation (grants
1527/07 and 196/08). Yinon Rudich acknowledges financial
support by the Helen and Martin Kimmel Award for Innovative
Investigation.},
abstract = {The Mediterranean region is expected to experience
substantial climatic change in the next 50 years. But,
possible effects of climate change on biogenic volatile
organic compound (VOC) emissions as well as on the formation
of secondary organic aerosols (SOA) produced from these VOC
are yet unexplored. To address such issues, the effects of
temperature on the VOC emissions of Mediterranean Holm Oak
and small Mediterranean stand of Wild Pistacio, Aleppo Pine,
and Palestine Oak have been studied in the Julich plant
aerosol atmosphere chamber. For Holm Oak the optical and
microphysical properties of the resulting SOA were
investigated.Monoterpenes dominated the VOC emissions from
Holm Oak $(97.5\%)$ and Mediterranean stand $(97\%).$ Higher
temperatures enhanced the overall VOC emission but with
different ratios of the emitted species. The amount of SOA
increased linearly with the emission strength with a
fractional mass yield of $6.0+/-0.6\%,$ independent of the
detailed emission pattern. The investigated particles were
highly scattering with no absorption abilities. Their
average hygroscopic growth factor of 1.13+/-0.03 at $90\%$
RH with a critical diameter of droplet activation was
100+/-4 nm at a supersaturation of $0.4\%.$ All
microphysical properties did not depend on the detailed
emission pattern, in accordance with an invariant O/C ratio
(0.57(+0.03/-0.1)) of the SOA observed by high resolution
aerosol mass spectrometry.The increase of Holm oak emissions
with temperature (approximate to $20\%$ per degree) was
stronger than e.g. for Boreal tree species (approximate to
$10\%$ per degree). The SOA yield for Mediterranean trees
determined here is similar as for Boreal trees. Increasing
mean temperature in Mediterranean areas could thus have a
stronger impact on BVOC emissions and SOA formation than in
areas with Boreal forests.},
keywords = {J (WoSType)},
cin = {IEK-8 / IBG-2},
ddc = {550},
cid = {I:(DE-Juel1)IEK-8-20101013 / I:(DE-Juel1)IBG-2-20101118},
pnm = {Atmosphäre und Klima},
pid = {G:(DE-Juel1)FUEK491},
shelfmark = {Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000280847700018},
doi = {10.5194/acp-10-7253-2010},
url = {https://juser.fz-juelich.de/record/12512},
}