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@ARTICLE{Huang:12600,
author = {Huang, C.C. and Winkler, R. G. and Sutmann, G. and Gompper,
G.},
title = {{S}emidilute {P}olymer {S}olutions at {E}quilibrium and
under {S}hear {F}low},
journal = {Macromolecules},
volume = {43},
issn = {0024-9297},
address = {Washington, DC},
publisher = {Soc.},
reportid = {PreJuSER-12600},
pages = {10107 - 10116},
year = {2010},
note = {The financial support by the Deutsche
Forschungsgemeinschaft (DFG) within SFB TR6 (project A4) is
gratefully acknowledged. We are grateful to the Julich
Supercomputer Centre (JSC) for allocation of a special
CPU-time grant.},
abstract = {The properties of semidilute polymer solutions are
investigated at equilibrium and under shear flow by
mesoscale simulations, which combine molecular dynamics
simulations and the multiparticle collision dynamics
approach. In semidilute solution, intermolecular
hydrodynamic and excluded volume interactions become
increasingly important due to the presence of polymer
overlap. At equilibrium, the dependence of the radius of
gyration, the structure factor, and the zero-shear viscosity
on the polymer concentration is determined and found to be
in good agreement with scaling predictions. In shear flow,
the polymer alignment and deformation are calculated as a
function of concentration. Shear thinning, which is related
to flow alignment and finite polymer extensibility, is
characterized by the shear viscosity and the normal stress
coefficients.},
keywords = {J (WoSType)},
cin = {IFF-2 / IAS-2 / JSC / JARA-HPC},
ddc = {540},
cid = {I:(DE-Juel1)VDB782 / I:(DE-Juel1)IAS-2-20090406 /
I:(DE-Juel1)JSC-20090406 / $I:(DE-82)080012_20140620$},
pnm = {BioSoft: Makromolekulare Systeme und biologische
Informationsverarbeitung (FUEK505) / Scientific Computing
(FUEK411) / 411 - Computational Science and Mathematical
Methods (POF2-411)},
pid = {G:(DE-Juel1)FUEK505 / G:(DE-Juel1)FUEK411 /
G:(DE-HGF)POF2-411},
shelfmark = {Polymer Science},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000284967000064},
doi = {10.1021/ma101836x},
url = {https://juser.fz-juelich.de/record/12600},
}