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@ARTICLE{Haanappel:12697,
author = {Haanappel, V. A. C. and Bär, B. and Tropartz, C. and
Mertens, J. and Tietz, F.},
title = {{V}arious {L}anthanum {F}errite-{B}ased {C}athode
{M}aterials {W}ith {N}i and {C}u {S}ubstitution for
{A}node-{S}upported {S}olid {O}xide {F}uel {C}ells},
journal = {Journal of fuel cell science and technology},
volume = {7},
issn = {1550-624X},
address = {New York, NY},
publisher = {ASME},
reportid = {PreJuSER-12697},
pages = {061017 - 061020},
year = {2010},
note = {Record converted from VDB: 12.11.2012},
abstract = {The electrochemical performance of solid oxide fuel cells
with cathodes made of La0.58Sr0.4Fe0.8Ni0.2O3-delta,
La0.58Sr0.4Fe0.8Cu0.2O3-delta,
La0.58Sr0.4Fe0.6Cu0.2Co0.2O3-delta,
La0.58Sr0.4Fe0.7Cu0.1Co0.2O3-delta, and La2Ni0.6Cu0.4O4 has
been investigated. As reference, electrochemical data from
cells with La0.58Sr0.4Co0.2Fe0.8O3-delta cathodes were taken
into account. The cathode layers were sintered at various
temperatures. After testing, cross-sectional analyses were
made in order to investigate microstructural changes in the
various layers. Electrochemical tests have shown that only
cells with a non-sintered Cu-containing cathode or with a
similar cathode treated with relatively low sintering
temperatures can be considered for SOFC applications.
However, it was clear that the tested cells with cathodes
including Cu and/or Ni showed electrochemical performance
which was always lower than that of reference cells with
La0.58Sr0.4Co0.2Fe0.8O3-delta cathode. No electrochemical
measurements were possible with cathodes sintered at or
above 1000 degrees C. Cross-sectional analyses revealed that
in all these cases the presence of Cu exhibited severe
chemical interaction with the electrolyte. In addition,
several undesired phases were formed in the cathode as well
as in the diffusion barrier layer. The extent of these
phases and the interaction with the electrolyte layer
increased with increasing sintering temperature. [DOI:
10.1115/1.4001355]},
keywords = {J (WoSType)},
cin = {IEK-PBZ / IEK-1 / IEK-3},
ddc = {620},
cid = {I:(DE-Juel1)IEK-PBZ-20101013 / I:(DE-Juel1)IEK-1-20101013 /
I:(DE-Juel1)IEK-3-20101013},
pnm = {Rationelle Energieumwandlung / SOFC - Solid Oxide Fuel Cell
(SOFC-20140602)},
pid = {G:(DE-Juel1)FUEK402 / G:(DE-Juel1)SOFC-20140602},
shelfmark = {Electrochemistry / Energy $\&$ Fuels},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000281307000017},
doi = {10.1115/1.4001355},
url = {https://juser.fz-juelich.de/record/12697},
}