000127637 001__ 127637 000127637 005__ 20230426083244.0 000127637 0247_ $$2arXiv$$aarXiv:1209.1923 000127637 0247_ $$2WOS$$aWOS:000308640300005 000127637 0247_ $$2doi$$a10.1103/PhysRevB.86.104416 000127637 0247_ $$2Handle$$a2128/4867 000127637 0247_ $$2MLZ$$aSabyasachiPMGDAIBC2012 000127637 0247_ $$2altmetric$$aaltmetric:2026089 000127637 037__ $$aFZJ-2012-00595 000127637 082__ $$a530 000127637 1001_ $$0P:(DE-HGF)0$$aSabyasachi, Sk.$$b0$$eCorresponding author 000127637 245__ $$aGlassy magnetic phase driven by short-range charge and magnetic ordering in nanocrystalline La1/3Sr2/3FeO3−δ: Magnetization, Mössbauer, and polarized neutron studies 000127637 260__ $$aCollege Park, Md.$$bAPS$$c2012 000127637 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1435819915_4339 000127637 3367_ $$2DataCite$$aOutput Types/Journal article 000127637 3367_ $$00$$2EndNote$$aJournal Article 000127637 3367_ $$2BibTeX$$aARTICLE 000127637 3367_ $$2ORCID$$aJOURNAL_ARTICLE 000127637 3367_ $$2DRIVER$$aarticle 000127637 500__ $$a10 pages, 9 figures. Fig. 1 available upon request or in http://www.ffn.ub.es/oscar/Articles.html. Accepted in Phys. Rev. B 000127637 520__ $$aThe charge ordered La$_{1/3}$Sr$_{2/3}$FeO$_{3-delta}$ (LSFO) in bulk and nanocrystalline forms are investigated using ac and dc magnetization, M'{o}ssbauer, and polarised neutron studies. A complex scenario of short range charge and magnetic ordering is realized from the polarised neutron studies in nanocrystalline specimen. This short range ordering does not involve any change in spin state and modification in the charge disproportion between Fe$^{3+}$ and Fe$^{5+}$ compared to bulk counterpart as evident in the M'{o}ssbauer results. The refinement of magnetic diffraction peaks provides magnetic moments of Fe$^{3+}$ and Fe$^{5+}$ are about 3.15$mu_B$ and 1.57$mu_B$ for bulk, and 2.7$mu_B$ and 0.53$mu_B$ for nanocrystalline specimen, respectively. The destabilization of charge ordering leads to magnetic phase separation, giving rise to the robust exchange bias (EB) effect. Strikingly, EB field at 5 K attains a value as high as 4.4 kOe for average size $sim$ 70 nm, which is zero for the bulk counterpart. A strong frequency dependence of ac susceptibility reveals cluster-glass like transition around $sim$ 65 K, below which EB appears. Overall results propose that finite size effect directs the complex glassy magnetic behavior driven by unconventional short range charge and magnetic ordering, and magnetic phase separation appears in nanocrystalline LSFO. 000127637 536__ $$0G:(DE-HGF)POF2-422$$a422 - Spin-based and quantum information (POF2-422)$$cPOF2-422$$fPOF II$$x0 000127637 536__ $$0G:(DE-HGF)POF2-424$$a424 - Exploratory materials and phenomena (POF2-424)$$cPOF2-424$$fPOF II$$x1 000127637 536__ $$0G:(DE-HGF)POF2-54G24$$a54G - JCNS (POF2-54G24)$$cPOF2-54G24$$fPOF II$$x2 000127637 536__ $$0G:(DE-HGF)POF2-544$$a544 - In-house Research with PNI (POF2-544)$$cPOF2-544$$fPOF II$$x3 000127637 542__ $$2Crossref$$i2012-09-12$$uhttp://link.aps.org/licenses/aps-default-license 000127637 588__ $$aDataset connected to 000127637 65027 $$0V:(DE-MLZ)SciArea-170$$2V:(DE-HGF)$$aMagnetism$$x0 000127637 65017 $$0V:(DE-MLZ)GC-2004-2016$$2V:(DE-HGF)$$aBasic research$$x2 000127637 65017 $$0V:(DE-MLZ)GC-180$$2V:(DE-HGF)$$aOthers$$x1 000127637 65017 $$0V:(DE-MLZ)GC-150$$2V:(DE-HGF)$$aNano Science and Technology $$x0 000127637 693__ $$0EXP:(DE-MLZ)DNS-20140101$$1EXP:(DE-MLZ)FRMII-20140101$$5EXP:(DE-MLZ)DNS-20140101$$6EXP:(DE-MLZ)NL6S-20140101$$aForschungs-Neutronenquelle Heinz Maier-Leibnitz $$eDNS: Diffuse scattering neutron time of flight spectrometer$$fNL6S$$x0 000127637 7001_ $$0P:(DE-HGF)0$$aPatra, M.$$b1 000127637 7001_ $$0P:(DE-HGF)0$$aMajumdar, S.$$b2 000127637 7001_ $$0P:(DE-HGF)0$$aGiri, S.$$b3 000127637 7001_ $$0P:(DE-HGF)0$$aDas, S.$$b4 000127637 7001_ $$0P:(DE-HGF)0$$aAmaral, V. 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