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@ARTICLE{Sabyasachi:127637,
author = {Sabyasachi, Sk. and Patra, M. and Majumdar, S. and Giri, S.
and Das, S. and Amaral, V. S. and Iglesias, O. and Borghols,
W. and Chatterji, T.},
title = {{G}lassy magnetic phase driven by short-range charge and
magnetic ordering in nanocrystalline
{L}a1/3{S}r2/3{F}e{O}3−δ: {M}agnetization, {M}össbauer,
and polarized neutron studies},
journal = {Physical review / B},
volume = {86},
number = {10},
issn = {1098-0121},
address = {College Park, Md.},
publisher = {APS},
reportid = {FZJ-2012-00595},
pages = {104416},
year = {2012},
note = {10 pages, 9 figures. Fig. 1 available upon request or in
http://www.ffn.ub.es/oscar/Articles.html. Accepted in Phys.
Rev. B},
abstract = {The charge ordered La$_{1/3}$Sr$_{2/3}$FeO$_{3-delta}$
(LSFO) in bulk and nanocrystalline forms are investigated
using ac and dc magnetization, M'{o}ssbauer, and polarised
neutron studies. A complex scenario of short range charge
and magnetic ordering is realized from the polarised neutron
studies in nanocrystalline specimen. This short range
ordering does not involve any change in spin state and
modification in the charge disproportion between Fe$^{3+}$
and Fe$^{5+}$ compared to bulk counterpart as evident in the
M'{o}ssbauer results. The refinement of magnetic diffraction
peaks provides magnetic moments of Fe$^{3+}$ and Fe$^{5+}$
are about 3.15$mu_B$ and 1.57$mu_B$ for bulk, and 2.7$mu_B$
and 0.53$mu_B$ for nanocrystalline specimen, respectively.
The destabilization of charge ordering leads to magnetic
phase separation, giving rise to the robust exchange bias
(EB) effect. Strikingly, EB field at 5 K attains a value as
high as 4.4 kOe for average size $sim$ 70 nm, which is zero
for the bulk counterpart. A strong frequency dependence of
ac susceptibility reveals cluster-glass like transition
around $sim$ 65 K, below which EB appears. Overall results
propose that finite size effect directs the complex glassy
magnetic behavior driven by unconventional short range
charge and magnetic ordering, and magnetic phase separation
appears in nanocrystalline LSFO.},
cin = {JARA-FIT / JCNS-2 / JCNS (München) ; Jülich Centre for
Neutron Science JCNS (München) ; JCNS-FRM-II},
ddc = {530},
cid = {$I:(DE-82)080009_20140620$ / I:(DE-Juel1)JCNS-2-20110106 /
I:(DE-Juel1)JCNS-FRM-II-20110218},
pnm = {422 - Spin-based and quantum information (POF2-422) / 424 -
Exploratory materials and phenomena (POF2-424) / 54G - JCNS
(POF2-54G24) / 544 - In-house Research with PNI (POF2-544)},
pid = {G:(DE-HGF)POF2-422 / G:(DE-HGF)POF2-424 /
G:(DE-HGF)POF2-54G24 / G:(DE-HGF)POF2-544},
experiment = {EXP:(DE-MLZ)DNS-20140101},
typ = {PUB:(DE-HGF)16},
eprint = {1209.1923},
howpublished = {arXiv:1209.1923},
archivePrefix = {arXiv},
SLACcitation = {$\%\%CITATION$ = $arXiv:1209.1923;\%\%$},
UT = {WOS:000308640300005},
doi = {10.1103/PhysRevB.86.104416},
url = {https://juser.fz-juelich.de/record/127637},
}