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@BOOK{Wenzel:128366,
author = {Wenzel, David},
title = {{K}eramiken und {K}eramikkombinationen zur
{F}einstpartikelabscheidung mit {H}ilfe thermischinduzierter
{P}otentialfelder und {E}lektronenemissionen},
volume = {152},
school = {RWTH Aachen},
type = {Dr.},
address = {Jülich},
publisher = {Forschungszentrum Jülich GmbH Zentralbibliothek, Verlag},
reportid = {FZJ-2013-00105},
isbn = {978-3-89336-820-4},
series = {Schriften des Forschungszentrums Jülich : Energie $\&$
Umwelt / Energy $\&$ Environment},
pages = {155 pp.},
year = {2012},
note = {Schriften des Forschungszentrums Jülich; RWTH Aachen,
Diss., 2012},
abstract = {Fine particle removal is an important step in coal or
biomass gasification and in advanced coal fired power plants
using PPCC-, IGCC- or oxycoal technology. Decreasing
pressure or temperature of the flue gas, as is necessary for
conventional ceramic candle filters, decreases the
thermodynamic efficiency and should therefore be avoided. In
this dissertation, which traces back to the AiF-project 275
Z, the electrochemical properties of several ceramic
materials and ceramic material combinations were
investigated. Based on those prior works aluminum oxide,
cerium oxide, chromium oxide, magnesium oxide, and zirconium
oxide were chosen for further investigation. Additional
measurements were performed on titanium dioxide, silicon
carbide and the chromium aluminum oxide/zirconium oxide
ceramic SEPR. Conductivity and charge carriers were
determined for temperatures between 800 °C and 1500 °C by
impedance spectroscopy measurements. The strength of the
electrostatic potentials between the ceramic materials were
also measured in this temperature range. The electron work
functions of the ceramics were determined by measuring the
conductivity between two electrodes, which was influenced by
the number of thermally emitted electrons. Ceramic samples
were used in an experiment conducted together with the
Karlsruhe Institute of Technology (KIT). In this experiment
titanium dioxide particles in a hot aerosol were thermally
charged, using those ceramic samples, and finally removed
using electrical fields. The electrical charge of the
particles and the efficiency of their removal were probed in
this experiment for temperatures between 900 °C and 1300
°C. The thermal emission of electrons from the ceramic
samples was also influenced by additional electric fields.
Using either silicon carbide or a ceramic combination of
aluminum oxide and zirconium oxide showed the best results.
Ceramics including chromium oxide might therefore not be
necessary for future applications of the thermionic
electrical filter, which was developed together with the KIT
and the Institute of Energy and Environmental Technology
e.V. (IUTA), so that problematic chromium(VI) emissions
would be avoidable.},
cin = {IEK-2},
cid = {I:(DE-Juel1)IEK-2-20101013},
pnm = {112 - Concentrating Solar Systems (POF2-112)},
pid = {G:(DE-HGF)POF2-112},
typ = {PUB:(DE-HGF)3},
url = {https://juser.fz-juelich.de/record/128366},
}