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@BOOK{Schlehuber:136214,
      author       = {Schlehuber, Dominic},
      title        = {{S}auerstofftransport und {D}egradationsverhalten von
                      {H}ochtemperaturmembranen für {CO}$_{2}$-freie
                      {K}raftwerke},
      volume       = {65},
      school       = {RWTH Aachen},
      type         = {Dr.},
      address      = {Jülich},
      publisher    = {Forschungszentrum Jülich GmbH Zentralbibliothek, Verlag},
      reportid     = {PreJuSER-136214},
      isbn         = {978-3-89336-630-9},
      series       = {Schriften des Forschungszentrums Jülich. Reihe Energie und
                      Umwelt / Energy und Environment},
      pages        = {VII, 139 S.},
      year         = {2010},
      note         = {Record converted from JUWEL: 18.07.2013; RWTH Aachen,
                      Diss., 2010},
      abstract     = {This thesis deals with membranes for oxygen separation from
                      air for high temperature application in fossil power plants
                      within the scope of the oxyfuel-process. Different
                      perovskite membrane materials (ABO$_{3- \delta}$) were
                      investigated concerning the oxygen transport and their
                      chemical stability under operation condition. The
                      association between oxygen transport properties and both the
                      thermodynamic boundary conditions as well as the material
                      properties (membrane thickness and surface properties) was
                      studied. One possibility to achieve higher oxygen fluxes
                      through the membrane is to reduce the thickness. In this
                      case the influence of surface processes on the overall
                      permeation becomes noteworthy. The effect of different
                      membrane surface modifications on the permeation rate was
                      investigated. For example it could be confirmed, that a
                      porous layer on the membrane surface significantly increases
                      the permeation flux due to the compensation of surface
                      exchange limitations. Beyond that, degradation processes
                      during the operation under power plant condition were
                      investigated. Special attention was attached to the
                      influence of degradation on the permeation flux during long
                      term operation. Thereby kinetic demixing of the membrane
                      material was observed.},
      cin          = {IEF / IEF-2},
      ddc          = {500},
      cid          = {I:(DE-Juel1)VDB1115 / I:(DE-Juel1)VDB810},
      shelfmark    = {EBA - Energy production, energy technology / EBA -
                      Energieerzeugung, Energietechnologie},
      typ          = {PUB:(DE-HGF)3},
      url          = {https://juser.fz-juelich.de/record/136214},
}