% IMPORTANT: The following is UTF-8 encoded. This means that in the presence
% of non-ASCII characters, it will not work with BibTeX 0.99 or older.
% Instead, you should use an up-to-date BibTeX implementation like “bibtex8” or
% “biber”.
@ARTICLE{Kornely:137158,
author = {Kornely, M. and Menzler, N. H. and Weber, A. and
Ivers-Tiffée, E.},
title = {{D}egradation of a {H}igh {P}erformance {SOFC} {C}athode by
{C}r-{P}oisoning at {OCV}-{C}onditions},
journal = {Fuel cells},
volume = {13},
number = {4},
issn = {1615-6846},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2013-03627},
pages = {506 - 510},
year = {2013},
abstract = {In this work we investigate the effect of Cr-poisoning at
OCV-condition by means of electrochemical impedance
spectroscopy (EIS). The anode-supported cell (ASC) is
operated in Cr-free environment for the first 70 h of the
cell test at 800 °C supplying air to the cathode and a
varying mixture of H2O/H2 to the anode. The performance of
the cell is determined by current-voltage (CV) measurement
after the start up. After an operating time of 70 h in the
absence of chromium species a Cr-source was switched on by
passing the oxidant (air) through a Crofer22APU powder bed.
In order to determine the degradation caused by Cr-poisoning
electrical impedance spectra are collected at every 29 h
of operating time. After further 275 h at OCV-condition in
the presence of Cr-source another CV-curve is measured. A
detailed analysis of the measured impedance spectra by the
distribution of relaxation times (DRT) enables a separation
of the cathode polarization resistance. During the Cr-free
operation the cathode polarization shows a constant value.
After the Cr-source is switched on a strong increase of the
cathode polarization resistance is observed. This unique
result shows clearly that Cr-poisoning of an
LSM/8YSZ-cathode already takes place at OCV-condition.},
cin = {IEK-1},
ddc = {620},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {123 - Fuel Cells (POF2-123) / SOFC - Solid Oxide Fuel Cell
(SOFC-20140602)},
pid = {G:(DE-HGF)POF2-123 / G:(DE-Juel1)SOFC-20140602},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000327706700007},
doi = {10.1002/fuce.201200182},
url = {https://juser.fz-juelich.de/record/137158},
}