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@ARTICLE{Fuchs:13753,
author = {Fuchs, H. and Brauers, T. and Dorn, H.-P. and Harder, H.
and Häseler, R. and Hofzumahaus, A. and Holland, F. and
Kanaya, Y. and Kajii, Y. and Kubistin, D. and Lou, S. and
Martinez, M. and Miyamoto, K. and Nishida, S. and Rudolf, M.
and Schlosser, E. and Wahner, A. and Yoshino, A. and
Schurath, U.},
title = {{T}echnical {N}ote: {F}ormal blind intercomparison of {HO}2
measurements in the atmosphere simulation chamber {SAPHIR}
during the {HO}x{C}omp campaign},
journal = {Atmospheric chemistry and physics},
volume = {10},
issn = {1680-7316},
address = {Katlenburg-Lindau},
publisher = {EGU},
reportid = {PreJuSER-13753},
pages = {12233 - 12250},
year = {2010},
note = {This work was supported by the EU FP-6 program EUROCHAMP
(grant no. RII3-CT-2004-505968) and ACCENT (Priority
1.1.6.3. Global Change and Ecosystems, grant no.
GOCE-CT-2004-505337).},
abstract = {Hydroperoxy radical (HO2) concentrations were measured
during the formal blind intercomparison campaign HOxComp
carried out in Julich, Germany, in 2005. Three instruments
detected HO2 via chemical conversion to hydroxyl radicals
(OH) and subsequent detection of the sum of OH and HO2 by
laser induced fluorescence (LIF). All instruments were based
on the same detection and calibration scheme. Because
measurements by a MIESR instrument failed during the
campaign, no absolute reference measurement was available,
so that the accuracy of individual instruments could not be
addressed. Instruments sampled ambient air for three days
and were attached to the atmosphere simulation chamber
SAPHIR during the second part of the campaign. Six
experiments of one day each were conducted in SAPHIR, where
air masses are homogeneously mixed, in order to investigate
the performance of instruments and to determine potential
interferences of measurements under well-controlled
conditions. Linear correlation coefficients (R-2) between
measurements of the LIF instruments are generally high and
range from 0.82 to 0.98. However, the agreement between
measurements is variable. The regression analysis of the
entire data set of measurements in SAPHIR yields slopes
between 0.69 to 1.26 and intercepts are smaller than typical
atmospheric daytime concentrations (less than 1 pptv). The
quality of fit parameters improves significantly, when data
are grouped into data subsets of similar water vapor
concentrations. Because measurements of LIF instruments were
corrected for a well-characterized water dependence of their
sensitivities, this indicates that an unknown factor related
to water vapor affected measurements in SAPHIR. Measurements
in ambient air are also well-correlated, but regression
parameters differ from results obtained from SAPHIR
experiments. This could have been caused by differences in
HO2 concentrations in the sampled air at the slightly
different locations of instruments.},
keywords = {J (WoSType)},
cin = {IEK-8},
ddc = {550},
cid = {I:(DE-Juel1)IEK-8-20101013},
pnm = {Atmosphäre und Klima},
pid = {G:(DE-Juel1)FUEK491},
shelfmark = {Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000285581000013},
doi = {10.5194/acp-10-12233-2010},
url = {https://juser.fz-juelich.de/record/13753},
}