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000138419 1001_ $$0P:(DE-HGF)0$$aLiu, Yaqing$$b0
000138419 245__ $$aTransistor Functions Based on Electrochemical Rectification
000138419 260__ $$aWeinheim$$bWiley-VCH$$c2013
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000138419 520__ $$aElectronic elements built from organic semiconductors, such as molecular transistors, have significant potential for technical innovations and mass use owing to their flexible mechanical properties, cost-effective processability, and tuneable optical properties.1 Self-assembled monolayer field-effect transistors (SAMFET) are among the latest developments of novel microelectronic devices.2 In SAMFETs, charge carriers laterally pass through a molecular layer (parallel to substrate) and exhibit transistor behavior, which can be modulated by an electrostatic gate. The charge transport properties of the SAMFETs are affected by the length of the channel.3, 4 Herein, we present a novel chip-based molecular transistor concept, which is based on charge-transfer processes across a monolayer of molecules perpendicular to the sample surface plane. To this end, redox active molecules are adsorbed to a collector electrode (CE) acting as electron-transfer mediators. A two-step charge transfer between solid interdigitated array electrodes (IDA), charge transfer mediator, and liquid-phase redox probe yields a unidirectional current response. An adsorbate-free generator electrode (GE) can be used to modulate the unidirectional currents, resulting in a transistor-like behavior. The electrochemical transistor-like system exhibits high current outputs at a low-voltage operation, high on/off switching current ratios, and is operated as a 24-bit code generator.
000138419 536__ $$0G:(DE-HGF)POF2-453$$a453 - Physics of the Cell (POF2-453)$$cPOF2-453$$fPOF II$$x0
000138419 536__ $$0G:(DE-HGF)POF2-423$$a423 - Sensorics and bioinspired systems (POF2-423)$$cPOF2-423$$fPOF II$$x1
000138419 588__ $$aDataset connected to CrossRef, juser.fz-juelich.de
000138419 7001_ $$0P:(DE-Juel1)128745$$aWolfrum, Bernhard$$b1$$ufzj
000138419 7001_ $$0P:(DE-Juel1)128689$$aHüske, Martin$$b2$$ufzj
000138419 7001_ $$0P:(DE-Juel1)128713$$aOffenhäusser, Andreas$$b3$$ufzj
000138419 7001_ $$0P:(DE-HGF)0$$aWang, Erkang$$b4
000138419 7001_ $$0P:(DE-Juel1)128707$$aMayer, Dirk$$b5$$eCorresponding author$$ufzj
000138419 773__ $$0PERI:(DE-600)2011836-3$$a10.1002/anie.201207778$$gVol. 52, no. 14, p. 4029 - 4032$$n14$$p4029 - 4032$$tAngewandte Chemie / International edition$$v52$$x1433-7851$$y2013
000138419 8564_ $$uhttps://juser.fz-juelich.de/record/138419/files/FZJ-2013-04550_PV.pdf$$yRestricted$$zPublished final document.
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000138419 9132_ $$0G:(DE-HGF)POF3-559H$$1G:(DE-HGF)POF3-550$$2G:(DE-HGF)POF3-500$$aDE-HGF$$bKey Technologies$$lBioSoft – Fundamentals for future Technologies in the fields of Soft Matter and Life Sciences$$vAddenda$$x0
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