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@ARTICLE{Liu:138419,
      author       = {Liu, Yaqing and Wolfrum, Bernhard and Hüske, Martin and
                      Offenhäusser, Andreas and Wang, Erkang and Mayer, Dirk},
      title        = {{T}ransistor {F}unctions {B}ased on {E}lectrochemical
                      {R}ectification},
      journal      = {Angewandte Chemie / International edition},
      volume       = {52},
      number       = {14},
      issn         = {1433-7851},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2013-04550},
      pages        = {4029 - 4032},
      year         = {2013},
      abstract     = {Electronic elements built from organic semiconductors, such
                      as molecular transistors, have significant potential for
                      technical innovations and mass use owing to their flexible
                      mechanical properties, cost-effective processability, and
                      tuneable optical properties.1 Self-assembled monolayer
                      field-effect transistors (SAMFET) are among the latest
                      developments of novel microelectronic devices.2 In SAMFETs,
                      charge carriers laterally pass through a molecular layer
                      (parallel to substrate) and exhibit transistor behavior,
                      which can be modulated by an electrostatic gate. The charge
                      transport properties of the SAMFETs are affected by the
                      length of the channel.3, 4 Herein, we present a novel
                      chip-based molecular transistor concept, which is based on
                      charge-transfer processes across a monolayer of molecules
                      perpendicular to the sample surface plane. To this end,
                      redox active molecules are adsorbed to a collector electrode
                      (CE) acting as electron-transfer mediators. A two-step
                      charge transfer between solid interdigitated array
                      electrodes (IDA), charge transfer mediator, and liquid-phase
                      redox probe yields a unidirectional current response. An
                      adsorbate-free generator electrode (GE) can be used to
                      modulate the unidirectional currents, resulting in a
                      transistor-like behavior. The electrochemical
                      transistor-like system exhibits high current outputs at a
                      low-voltage operation, high on/off switching current ratios,
                      and is operated as a 24-bit code generator.},
      cin          = {ICS-8 / PGI-8 / JARA-FIT},
      ddc          = {540},
      cid          = {I:(DE-Juel1)ICS-8-20110106 / I:(DE-Juel1)PGI-8-20110106 /
                      $I:(DE-82)080009_20140620$},
      pnm          = {453 - Physics of the Cell (POF2-453) / 423 - Sensorics and
                      bioinspired systems (POF2-423)},
      pid          = {G:(DE-HGF)POF2-453 / G:(DE-HGF)POF2-423},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000316915500043},
      pubmed       = {pmid:23460501},
      doi          = {10.1002/anie.201207778},
      url          = {https://juser.fz-juelich.de/record/138419},
}