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@PHDTHESIS{Morgan:141552,
author = {Morgan, Caitlin},
title = {{M}agnetoresistance and transport in carbon nanotube-based
devices},
volume = {78},
school = {Universität Duisburg},
type = {Dissertation},
address = {Jülich},
publisher = {Forschungszentrum Jülich GmbH Zentralbibliothek, Verlag},
reportid = {FZJ-2013-06719},
isbn = {978-3-89336-926-3},
series = {Schriften des Forschungszentrums Jülich. Reihe
Schlüsseltechnologien / key technologies},
pages = {VIII, 131 S.},
year = {2013},
note = {Dissertation, Universität Duisburg, 2013},
abstract = {In addition to exhibiting ballistic transport, the low
atomic number and low abundance of $^{13}$C spin nuclei in
CNTs lead to low spin orbit coupling [1, 2] and hyperfine
interaction, indicating a long spin dephasing length. This
makes CNTs a material of interest in spintronics, where
injecting a spin-polarized current from a ferromagnetic lead
into a nonmagnetic channel presents an ongoing challenge. As
typical ferromagnetic materials form unreliable contact to
CNTs [3, 4, 5], we investigate a novel contact material, the
alloy CoPd. We thus combine the stable ohmic contact Pd
forms to CNTs [6] and the high polarization of Co and
Co-based alloys [7]. This work begins with a
characterization of the material CoPd to find the optimal
alloy composition. When grown on an SiO$_{2}$ surface, CoPd
is shown to have both surface and interfacial roughness of
less than 0.5 nm. Magnetically, extended films of CoPd
exhibit a complicated behavior with a large out-of-plane
component manifesting itself in bubble and stripe domains.
However, arrays of fabricated nanostructures of CoPd show a
clear in-plane easy axis with little or no out-of-plane
component and a high saturation magnetization. Lastly,
electrical measurements performed in CoPd-contacted CNTs
indicate the formation of highly transparent ohmic contacts.
The best performance was found with the alloy
Co$_{50}$Pd$_{50}$. Local magnetoresistance (MR)
measurements show a dependence on the contact geometry,
temperature, and the electronic structure of the CNT.
Devices with nanostructured contacts resulted in precise,
reliable switching. The magnitude of local MR was shown to
increase with lower temperatures and in devices where a
stronger tunnel barrier was present. CNTs intrinsically form
tunnel barriers at low temperatures, and the strength
depends on the contact interface, although it may be
suppressed and enhanced via tuning of the bias and gate
voltages. Finally, nonlocal three-terminal measurements were
performed. While the signal in local measurements may be
enhanced by effects such as anisotropic magnetoresistance
(AMR), Hall efects, and various local ohmic effects,
nonlocal measurements probe only the pure spin current, and
are proof that spin injection and detection occur in
CNT-based devices with CoPd contacts. Furthermore, Hanle
measurements showed a clear spin precession, with a spin
lifetime $\tau_{s}$ = 1.1 ns. In conclusion, we have
successfully demonstrated the occurrance of spin injection
and detection in CNTs contacted by CoPd. The system has all
the requirements of a spin valve device: highly polarized
leads, intrinsic tunnel barriers, and transparent contact
resulting in efficient injection, a nanotube channel that
allows for a long spin lifetime, and reliable spin
detection, and can therefore provide much useful information
for the field of spintronics.},
keywords = {Dissertation (GND)},
cin = {PGI-6},
cid = {I:(DE-Juel1)PGI-6-20110106},
pnm = {422 - Spin-based and quantum information (POF2-422)},
pid = {G:(DE-HGF)POF2-422},
typ = {PUB:(DE-HGF)3 / PUB:(DE-HGF)11},
url = {https://juser.fz-juelich.de/record/141552},
}