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000001445 084__ $$2WoS$$aMeteorology & Atmospheric Sciences
000001445 1001_ $$0P:(DE-Juel1)2693$$aBohn, B.$$b0$$uFZJ
000001445 245__ $$aPhotolysis frequency measurement techniques: results of a comparison within the ACCENT project
000001445 260__ $$aKatlenburg-Lindau$$bEGU$$c2008
000001445 300__ $$a5373 - 5391
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000001445 440_0 $$09601$$aAtmospheric Chemistry and Physics$$v8$$x1680-7316$$y17
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000001445 520__ $$aAn intercomparison of different radiometric techniques measuring atmospheric photolysis frequencies j(NO2), j(HCHO) and j((OD)-D-1) was carried out in a two-week field campaign in June 2005 at Julich. Germany. Three double-monochromator based spectroradiometers (DM-SR), three single-monochromator based spectroradiometers with diode-array detectors (SM-SR) and seventeen filter radiometers (FR) (ten j(NO2))-FR, seven j((OD)-D-1)-FR) took part in this comparison. For j(NO2), all spectroradiometer results agreed within +/- 3%. For j(HCHO), agreement was slightly poorer between -8% and +4% of the DM-SR reference result. For the SM-SR deviations were explained by poorer spectral resolutions and lower accuracies caused by decreased sensitivities of the photodiode arrays in a wave-length range below 350 nm. For j((OD)-D-1), the results were more complex within +8% and -4% with increasing deviations towards larger solar zenith angles for the SM-SR. The direction and the magnitude of the deviations were dependent on the technique of background determination. All j(NO2))-FR showed good linearity with sing-le calibration factors being sufficient to convert from output voltages to j(NO2)). Measurements were feasible until sunset and comparison with previous calibrations showed good long-term stability. For the j((OD)-D-1)-FR, conversion from output voltages to j((OD)-D-1) needed calibration factors and correction functions considering the influences of total ozone column and elevation of the sun. All instruments showed good linearity at photolysis frequencies exceeding about 10% of maximum values. At larger solar zenith angles, the agreement was non-uniform with deviations explainable by insufficient correction functions. Comparison with previous calibrations for sonic J((OD)-D-1)-FR indicated drifts of calibration factors.
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000001445 7001_ $$0P:(DE-HGF)0$$aCorlett, G.K.$$b1
000001445 7001_ $$0P:(DE-HGF)0$$aGillmann, M.$$b2
000001445 7001_ $$0P:(DE-HGF)0$$aSanghavi, S.$$b3
000001445 7001_ $$0P:(DE-HGF)0$$aStange, G.$$b4
000001445 7001_ $$0P:(DE-HGF)0$$aTensing, E.$$b5
000001445 7001_ $$0P:(DE-HGF)0$$aVrekoussis, M.$$b6
000001445 7001_ $$0P:(DE-HGF)0$$aBloss, W. J.$$b7
000001445 7001_ $$0P:(DE-HGF)0$$aClapp, L.J.$$b8
000001445 7001_ $$0P:(DE-HGF)0$$aKortner, M.$$b9
000001445 7001_ $$0P:(DE-Juel1)16317$$aDorn, H.-P.$$b10$$uFZJ
000001445 7001_ $$0P:(DE-HGF)0$$aMonks, P. S.$$b11
000001445 7001_ $$0P:(DE-HGF)0$$aPlatt, U.$$b12
000001445 7001_ $$0P:(DE-HGF)0$$aPlass-Dülmer, C.$$b13
000001445 7001_ $$0P:(DE-HGF)0$$aMihalopoulos, N.$$b14
000001445 7001_ $$0P:(DE-HGF)0$$aHeard, D. E.$$b15
000001445 7001_ $$0P:(DE-HGF)0$$aClemitshaw, K. C.$$b16
000001445 7001_ $$0P:(DE-HGF)0$$aMeixner, F. X.$$b17
000001445 7001_ $$0P:(DE-HGF)0$$aPrevot, A. S. H.$$b18
000001445 7001_ $$0P:(DE-HGF)0$$aSchmitt, R.$$b19
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