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@PHDTHESIS{Kamil:150523,
author = {Kamil, Sladek},
title = {{R}ealization of {III}-{V} semiconductor nano structures
towards more efficient (opto-) electronic devices},
school = {RWTH Aachen},
type = {Dr.},
address = {Jülich},
publisher = {PGI-9: Halbleiter-Nanoelektronik},
reportid = {FZJ-2014-00577},
pages = {100},
year = {2013},
note = {RWTH Aachen, Diss., 2013},
abstract = {Solid state electronics and their application in personal
computers, smartphones, digital cameras and entertainment
devices (to name a few) have gained such a rapid progress
that it’s already barely imaginable how our future
technological environment will evolve in the next few years.
In parallel, however, concerns about excessive use of the
world’s limited natural energy resources has led to a
rethinking with respect to the design and production of
future electronics. One of the most promising solutions to
further improve the efficiency of electronics is the
combination of the well established silicon technology with
III-V semiconductor nano structures which have been
extensively investigated in various fields for the last few
decades. InAs nano structures, in particular, are
intrinsically conductive due to their characteristic
conduction band profile, caused by surface states. The
materials high bulk carrier mobility gives rise to expect a
significant boost in efficiency of electronic devices that
employ InAs nano structures. In this work, three different
aspects of device improvement are addressed: the exchange of
channel material in traditional CMOS, the development of new
nanostructure based concepts and the use of direct band gap
properties for more cost-effective sensing devices. The
established SA MOVPE of III-V nano structures on III-V
substrates serves as a starting point. Systematic
experiments are conducted in order to address several
significant questions regarding the suitability of III-V
nano structures as building blocks for future electronic
devices. It is found that a large variety of free-standing
InAs nanowires with different properties can be produced in
an ordered and controlled fashion. The results show that
uniform InAs nanowires with a high aspect ratio can be
produced selectively on GaAs(111)B and GaAs(110) oriented
surfaces, the latter being also a natural cleaved edge
direction of industrially used Si(001) substrates. In
addition, very thin InAs nanowires with diameters down to 20
nm are obtained as a side effect on non-structured
cleaved-edge sidewalls of GaAs(001). N-type doping with
disilane is found to have a general impact on the nanowire
morphology, resulting in a reduced height vs. diameter
aspect ratio with an increased amount of doping applied
during deposition. It is observed that all wires exhibit an
intrinsic conductivity with an ohmic behavior which is
further increased after doping. Also, the nanowire diameter
is found to be a potential parameter to tune their
electronic properties. A series of experiments with
different growth parameters and the successive
characterization of the nanowires‘ crystal structure
reveal that different group-V partial pressures affect the
formation of stacking faults and the crystal‘s wurtzite to
zinc blende ratio. A significant step to combine the gained
knowledge on controlled bottom-up InAs nanowire fabrication
and benefits of SA MOVPE in N2 ambient with current silicon
technology is the transition of InAs growth to silicon
substrates. The technique of flow modulated epitaxy is
adopted from MOVPE growth in hydrogen ambient and adapted
and optimized for growth in N2 in order overcome the lack of
polarity on silicon. As a result, InAs nanowire growth on
Si(111) is carried out with a high yield of vertical wires.
After the investigation of free standing InAs nanowires
mainly for concepts exceeding CMOS, a methodology for the
deposition of lateral InAs nano structures on silicon by SA
MOVPE was presented, aimed towards the exchange of channel
material in current planar electronic devices. Growth
parameters adopted from GaAs/InAs core-shell nanowire growth
are applied to a variety of differently oriented and
patterned substrates. The obtained lateral structures are
characterized with respect to morphology, crystal structure
and electronic properties. High crystallinity and
conductivity are found and discussed in comparison to the
results obtained from vertical nanowires. Finally, quantum
cascade structures based on ternary III-V semiconductors
with high indium content are investigated with respect to
single mode emission for gas sensing applications. It is
found that curved laser waveguides are capable of single
mode emission which is explained by the interaction of
coupled cavities, resulting in strong side mode suppression.
The monolithic approach without need for complicated sample
processing has tremendous potential for the fabrication of
cost effective and portable gas sensing devices.},
keywords = {Dissertation (GND)},
cin = {PGI-9},
cid = {I:(DE-Juel1)PGI-9-20110106},
pnm = {421 - Frontiers of charge based Electronics (POF2-421)},
pid = {G:(DE-HGF)POF2-421},
typ = {PUB:(DE-HGF)11},
url = {https://juser.fz-juelich.de/record/150523},
}